ArticleScience advances2023
Achieving ideal transistor characteristics in conjugated polymer semiconductors.
Article in Science advances, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- A rubbery semiconducting heterojunction film for fully rubbery multiplexed near-infrared phototransistor arrays.Science advances · 2026Article
- High-Performance Air-Stable Polymer Monolayer Transistors for Monolithic 3D CMOS logics.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Highly oriented semiconducting polymer nanofilm with enhanced crystallinity.Nature communications · 2025Article
- Models connecting microstructure and charge transport in disordered semiconducting polymers: from theories to digital design.Materials horizons · 2025Review
- Surface-Engineered MoOMolecules (Basel, Switzerland) · 2025Article
- Constructing N-Containing Poly(p-Phenylene) (PPP) Films Through A Cathodic-Dehalogenation Polymerization Method.Small methods · 2024Article
- Modulation between capacitor and conductor for a redox-active 2D bis(terpyridine)cobalt(II) nanosheet via anion-exchange.Communications chemistry · 2024Article
- A Three-in-One Hybrid Strategy for High-Performance Semiconducting Polymers Processed from Anisole.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
Corrections and comments
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Authors and funding
25 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Organic thin-film transistors (OTFTs) with ideal behavior are highly desired, because nonideal devices may overestimate the intrinsic property and yield inferior performance in applications. In reality, most polymer OTFTs reported in the literature do not exhibit ideal characteristics. Supported by a structure-property relationship study of several low-disorder conjugated polymers, here, we present an empirical selection rule for polymer candidates for textbook-like OTFTs with high reliability factors (100% for ideal transistors). The successful candidates should have low energetic disorder along their backbones and form thin films with spatially uniform energetic landscapes. We demonstrate that these requirements are satisfied in the semicrystalline polymer PffBT4T-2DT, which exhibits a reliability factor (~100%) that is exceptionally high for polymer devices, rendering it an ideal candidate for OTFT applications. Our findings broaden the selection of polymer semiconductors with textbook-like OTFT characteristics and would shed light upon the molecular design criteria for next-generation polymer semiconductors.
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Registered trials
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