ArticleNature communications2023
Facile conversion of water to functional molecules and cross-linked polymeric films with efficient clusteroluminescence.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Polymer-constrained excimer enables flexible and self-healable optoelectronic elastomer for mechanical sensor.Nature communications · 2025Article
- Spontaneous amino-yne click polymerization enabled by pyridinium-activated alkynes toward p-π conjugated ionic polymers.Chemical science · 2025Article
- Water in Triple-Bond-Based Polymerizations: Roles as a Solvent or Monomer.Polymer science & technology (Washington, D.C.) · 2025Review
- Emergent clusteroluminescence from nonemissive molecules.Nature communications · 2025Review
- Water as a Reactant: DABCO-Catalyzed Hydration of Activated Alkynes for the Synthesis of Divinyl Ethers.The Journal of organic chemistry · 2024Article
- Narrowband clusteroluminescence with 100% quantum yield enabled by through-space conjugation of asymmetric conformation.Nature communications · 2024Article
- Recent Progress in Nonconventional Luminescent Macromolecules and their Applications.Macromolecules · 2024Review
- Article
- A Self-Assemble Supramolecular Film with Humidity Visualization Enabled by Clusteroluminescence.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Hydrogen-Bonding-Driven Nontraditional Photoluminescence of aMolecules (Basel, Switzerland) · 2023Article
Corrections and comments
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Authors and funding
6 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Exploring approaches to utilize abundant water to synthesize functional molecules and polymers with efficient clusteroluminescence properties is highly significant but has yet to be reported. Herein, a chemistry of water and alkyne is developed. The synthesized products are proven as nonaromatic clusteroluminogens that could emit visible light. Their emission colors and luminescent efficiency could be adjusted by manipulating through-space interaction using different starting materials. Besides, the free-standing polymeric films with much high photoluminescence quantum yields (up to 45.7%) are in situ generated via a water-involved interfacial polymerization. The interfacial polymerization-enhanced emission of the polymeric films is observed, where the emission red-shifts and efficiency increases when the polymerization time is prolonged. The synthesized polymeric film is also verified as a Janus film. It exhibits a vapor-triggered reversible mechanical response which could be applied as a smart actuator. Thus, this work develops a method to synthesize clusteroluminogens using water, builds a clear structure-property relationship of clusteroluminogens, and provides a strategy to in situ construct functional water-based polymeric films.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.