ArticlePolymers2023
Unlocking the Potential Use of Reactive POSS as a Coagent for EPDM/PP-Based TPV.
Article in Polymers, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Octavinyl-POSS as a Modifier of Thermoplastic Polyolefin Elastomers Based on Ethylene-Propylene-Diene and Ethylene-1-Octene EPDM/POEs Blends.Materials (Basel, Switzerland) · 2026Article
- Characterization of Mixtures Based on High-Density Polyethylene and Plasticized Starch.Polymers · 2024Article
- Ultraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management.Nature communications · 2023Article
- Combined Sulfur and Peroxide Vulcanization of Filled and Unfilled EPDM-Based Rubber Compounds.Materials (Basel, Switzerland) · 2023Article
Corrections and comments
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Authors and funding
5 authors.
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Abstract
Thermoplastic vulcanizates (TPVs) are multifunctional materials consisting of two or more phases with solid elastomeric properties at room temperatures and fluid-like properties above their melting point. They are produced through a reactive blending process known as dynamic vulcanization. The most widely produced TPV type is ethylene propylene diene monomer/polypropylene (EPDM/PP), which is the focus of this study. The peroxides are mainly selected to be used in crosslinking of EPDM/PP-based TPV. However, they still have some disadvantages, such as the side reactions resulting in the beta chain scission of the PP phase and undesired disproportionation reactions. To eliminate these disadvantages, coagents are used. In this study, for the first time, the use of vinyl functionalized polyhedral oligomeric silsesquioxane (OV-POSS) nanoparticles was investigated as a potential coagent in EPDM/PP-based TPV production via peroxide-initiated dynamic vulcanization. The properties of the TPVs having POSS were compared with the conventional TPVs containing conventional coagents, such as triallyl cyanurate (TAC). POSS content and EPDM/PP ratio were investigated as the material parameters. Mechanical properties of EPDM/PP TPVs exhibited higher values in the presence of OV-POSS, which resulted from the active participation of OV-POSS into the three-dimensional network structure of EPDM/PP during dynamic vulcanization.
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