ArticleNature communications2023
Three-dimensional covalent organic frameworks with pto and mhq-z topologies based on Tri- and tetratopic linkers.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed.
- Steering Electron Transport in Intrinsically Piezoelectric Covalent Organic Frameworks for Efficient COAngewandte Chemie (International ed. in English) · 2026Article
- Modulating Optoelectronic Properties of TBQP-Based Covalent Organic Frameworks for Chemical Sensing.ACS omega · 2026Article
- Reversible Bond Dynamics Enable Crystallinity-Healed COF Membranes for Selective Ion Transport.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Article
- Support field neural representation learner framework for learning stability landscapes in molecular geometry.npj biomedical innovations · 2025Article
- Confining Quantum Dots Within Covalent Organic Framework Cages for Coupled COAdvanced materials (Deerfield Beach, Fla.) · 2025Article
- Multi-Modal Topology-Aware Graph Neural Network for Robust Chemical-Protein Interaction Prediction.International journal of molecular sciences · 2025Article
- Steric effect of intermediates induces formation of three-dimensional covalent organic frameworks.Nature communications · 2025Article
- Integrating Multifunctionalities into a 3D Covalent Organic Framework for Efficient COAngewandte Chemie (International ed. in English) · 2025Article
- Synergistic experimental and computational investigation of azo-linked porphyrin-based porous organic polymers for CORSC advances · 2025Article
- Exploring chiral and achiral properties of novel multilayer 3D polymers: synthesis and characterization.RSC advances · 2025Article
- 3D N-heterocyclic covalent organic frameworks for urea photosynthesis from NHNature communications · 2025Article
- A General Synthesis Method for Covalent Organic Framework and Inorganic 2D Materials Hybrids.Precision chemistry · 2024Article
- Covalent Bonding of MXene/COF Heterojunction for Ultralong Cycling Li-Ion Battery Electrodes.Molecules (Basel, Switzerland) · 2024Article
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Authors and funding
13 authors.
Funding
Abstract
Three-dimensional (3D) covalent organic frameworks (COFs) possess higher surface areas, more abundant pore channels, and lower density compared to their two-dimensional counterparts which makes the development of 3D COFs interesting from a fundamental and practical point of view. However, the construction of highly crystalline 3D COF remains challenging. At the same time, the choice of topologies in 3D COFs is limited by the crystallization problem, the lack of availability of suitable building blocks with appropriate reactivity and symmetries, and the difficulties in crystalline structure determination. Herein, we report two highly crystalline 3D COFs with pto and mhq-z topologies designed by rationally selecting rectangular-planar and trigonal-planar building blocks with appropriate conformational strains. The pto 3D COFs show a large pore size of 46 Å with an extremely low calculated density. The mhq-z net topology is solely constructed from totally face-enclosed organic polyhedra displaying a precise uniform micropore size of 1.0 nm. The 3D COFs show a high CO
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