ArticleProceedings of the National Academy of Sciences of the United States of America2023
Dynamic orbital hybridization triggered spin-disorder renormalization via super-exchange interaction for oxygen evolution reaction.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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6 citing papers in PubMed, 60 citations in OpenAlex.
- Selenized Binary Transition Metals-MXene Composite for High-Performance Asymmetric Hybrid Capacitors.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Spin Effects in Optimizing Electrochemical Applications.ACS materials Au · 2025Review
- Spin effects in regulating the adsorption characteristics of metal ions.Chemical science · 2025Article
- Electron-phonon coupling and coherent energy superposition induce spin-sensitive orbital degeneracy for enhanced acidic water oxidation.Nature communications · 2025Article
- Spin polarization induced by atomic strain of MBene promotes the ·ONature communications · 2025Article
- Boosting oxygen evolution reaction by FeNi hydroxide-organic framework electrocatalyst toward alkaline water electrolyzer.Nature communications · 2024Article
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Authors and funding
9 authors at 5 institutions in 1 country.
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Abstract
The oxygen evolution reaction (OER) underpins many aspects of energy storage and conversion in modern industry and technology, but which still be suffering from the dilemma of sluggish reaction kinetics and poor electrochemical performance. Different from the viewpoint of nanostructuring, this work focuses on an intriguing dynamic orbital hybridization approach to renormalize the disordering spin configuration in porous noble-metal-free metal-organic frameworks (MOFs) to accelerate the spin-dependent reaction kinetics in OER. Herein, we propose an extraordinary super-exchange interaction to reconfigure the domain direction of spin nets at porous MOFs through temporarily bonding with dynamic magnetic ions in electrolytes under alternating electromagnetic field stimulation, in which the spin renormalization from disordering low-spin state to high-spin state facilitates rapid water dissociation and optimal carrier migration, leading to a spin-dependent reaction pathway. Therefore, the spin-renormalized MOFs demonstrate a mass activity of 2,095.1 A g
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