ArticleProceedings of the National Academy of Sciences of the United States of America2023
Distinguishing homogeneous advanced oxidation processes in bulk water from heterogeneous surface reactions in organic oxidation.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed.
- Self-Sustaining Ce(IV)/Ce(III) Cycle for Spontaneous Surface Hydroxyl Radical Generation.Environmental science & technology · 2026Article
- Selective Two-Electron Phenol Oxidation Polymerization for Water Purification.Angewandte Chemie (International ed. in English) · 2026Article
- In Situ Turning Pollutants Into Catalysts: A Phase-Transition Self-Catalysis Paradigm for Sustainable Water Treatment.Angewandte Chemie (International ed. in English) · 2026Article
- In situ iodine generation enables solution-phase polymerization of organic pollutants for continuous resource recovery from water.Nature communications · 2026Article
- Selective carbonate radicals generation via hydraulically driven piezo-catalysis for polymerization-based removal of phenolic pollutants.Nature communications · 2026Article
- Axial oxygen coordination drives spin-regulated electron transfer in single-atom Fe catalysts for selective pollutant transformation.Nature communications · 2026Article
- Defect-induced electric field effects direct Fenton-like oxidation pathways towards polymerization for sustainable water treatment.Nature communications · 2025Article
- Efficient phenol removal by δ-MnOiScience · 2025Article
- Non-negligible Organic Carbon Transfer during Organic Pollutant Degradation Processes by Advanced Oxidation Technologies.ACS environmental Au · 2025Review
- Intrinsic strain of defect sites steering chlorination reaction for water purification.Nature communications · 2025Article
- High-entropy alloys catalyzing polymeric transformation of water pollutants with remarkably improved electron utilization efficiency.Nature communications · 2025Article
- Coordination engineering of heterogeneous high-valent Fe(IV)-oxo for safe removal of pollutants via powerful Fenton-like reactions.Nature communications · 2024Article
- Long-lasting organics removal via •OH adsorbed transition metal flocs: Electron transfer-mediated H-bond and van der Waals force.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Recovering palladium and gold by peroxydisulfate-based advanced oxidation process.Science advances · 2024Article
- Carbon redirection via tunable Fenton-like reactions under nanoconfinement toward sustainable water treatment.Nature communications · 2024Article
- Tailoring d-band center of high-valent metal-oxo species for pollutant removal via complete polymerization.Nature communications · 2024Article
- Electronic structure modulation of iron sites with fluorine coordination enables ultra-effective HNature communications · 2024Article
- In situ ligand-modulated activation of inert Ce(III/IV) into ozonation catalyst for efficient water treatment.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
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6 authors.
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Abstract
Clarifying the reaction pathways at the solid-water interface and in bulk water solution is of great significance for the design of heterogeneous catalysts for selective oxidation of organic pollutants. However, achieving this goal is daunting because of the intricate interfacial reactions at the catalyst surface. Herein, we unravel the origin of the organic oxidation reactions with metal oxide catalysts, revealing that the radical-based advanced oxidation processes (AOPs) prevail in bulk water but not on the solid catalyst surfaces. We show that such differing reaction pathways widely exist in various chemical oxidation (e.g., high-valent Mn
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