ReviewChemical reviews2023
Mechanistic Insights Gained by High Spatial Resolution Reactivity Mapping of Homogeneous and Heterogeneous (Electro)Catalysts.
Review in Chemical reviews, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Who cites it
13 citing papers in PubMed.
- Electrochemiluminescence Imaging for In Situ Electrocatalysis Characterization: Recent Progress and Mechanistic Insights.Chemical & biomedical imaging · 2026Review
- Scanning Photoelectrochemical (Cell) Microscopy forChemical & biomedical imaging · 2026Review
- Building Chemistry from "Lego" Blocks: Metal-Organic Frameworks after the 2025 Nobel Prize.ACS central science · 2026Review
- Direction-resolved nanoscale optical imaging with near-nanometer resolution by emerging infrared torsional force microscopy.Nature communications · 2026Article
- Advancements in Understanding the Physicochemical Properties of Reticular Materials: An In Situ and Operando Spectroscopic Perspective.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Unveiling the Power of Proximity of Prevalent Fe-Based Tandem Catalysts in COChemical reviews · 2025Review
- Nanoscale Analysis of Sulfur Poisoning Effects on Hydrogen Sorption in Single Pd Nanoparticles.ACS nano · 2025Article
- Nanoscale Chemical Imaging of Basic Sites Distribution on Catalytically Active Mg-Al Mixed Oxide Particles.Chemical & biomedical imaging · 2025Article
- A Decade of Catalytic Progress in 1,4-Dihydropyridines (1,4-DHPs) Synthesis (2016-2024).Current organic synthesis · 2025Article
- Advances and challenges in dynamic photo-induced force microscopy.Discover nano · 2024Review
- Extracting the Heterogeneous 3D Structure of Molecular Films Using Higher Dimensional SFG Microscopy.The journal of physical chemistry letters · 2024Article
- Understanding Photo(electro)catalysts for Energy Conversion via Operando Functional Imaging.Chemical & biomedical imaging · 2023Review
- Nanoimaging of Facet-Dependent Adsorption, Diffusion, and Reactivity of Surface Ligands on Au Nanocrystals.Nano letters · 2023Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The recent development of high spatial resolution microscopy and spectroscopy tools enabled reactivity analysis of homogeneous and heterogeneous (electro)catalysts at previously unattainable resolution and sensitivity. These techniques revealed that catalytic entities are more heterogeneous than expected and local variations in reaction mechanism due to divergences in the nature of active sites, such as their atomic properties, distribution, and accessibility, occur both in homogeneous and heterogeneous (electro)catalysts. In this review, we highlight recent insights in catalysis research that were attained by conducting high spatial resolution studies. The discussed case studies range from reactivity detection of single particles or single molecular catalysts, inter- and intraparticle communication analysis, and probing the influence of catalysts distribution and accessibility on the resulting reactivity. It is demonstrated that multiparticle and multisite reactivity analyses provide unique knowledge about reaction mechanism that could not have been attained by conducting ensemble-based, averaging, spectroscopy measurements. It is highlighted that the integration of spectroscopy and microscopy measurements under realistic reaction conditions will be essential to bridge the gap between model-system studies and real-world high spatial resolution reactivity analysis.
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Registered trials
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