ArticleNature communications2023
Two-dimensional infrared-Raman spectroscopy as a probe of water's tetrahedrality.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Cell Viability, Drug Screening, and Mechanism Study Under Mild Phototherapy Integrated Chemotherapy (PIC).Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Magnetic Field-Driven Interface Hydroxylation via the Vibrational Stark Effect Boosts Alkaline Hydrogen Evolution Reaction.JACS Au · 2025Article
- Development of a Spectroscopic Map to Explain the Broad Raman Peak for Alkynes Solvated in Triethylamine.The journal of physical chemistry. B · 2025Article
- Investigating the Water State in Saccharide Solutions by Infrared/Far-Infrared Spectra in the 1000-100 cmThe journal of physical chemistry. A · 2025Article
- Paschen-Back effect modulation of SONature communications · 2025Article
- Dichotomous behavior of water in binary mixtures with a turning point between 40 and 60 °C.RSC advances · 2025Article
- Evidence for two kinds of hydrogen-bonding networks in ionic solutions by 2D infrared correlation spectroscopy.Scientific reports · 2025Article
- Experimental Access to Mode-Specific Coupling between Quantum Molecular Vibrations and Classical Bath Modes.The journal of physical chemistry letters · 2023Article
Corrections and comments
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Authors and funding
2 authors.
Funding
Abstract
Two-dimensional spectroscopic techniques combining terahertz (THz), infrared (IR), and visible pulses offer a wealth of information about coupling among vibrational modes in molecular liquids, thus providing a promising probe of their local structure. However, the capabilities of these spectroscopies are still largely unexplored due to experimental limitations and inherently weak nonlinear signals. Here, through a combination of equilibrium-nonequilibrium molecular dynamics (MD) and a tailored spectrum decomposition scheme, we identify a relationship between the tetrahedral order of liquid water and its two-dimensional IR-IR-Raman (IIR) spectrum. The structure-spectrum relationship can explain the temperature dependence of the spectral features corresponding to the anharmonic coupling between low-frequency intermolecular and high-frequency intramolecular vibrational modes of water. In light of these results, we propose new experiments and discuss the implications for the study of tetrahedrality of liquid water.
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