Evidence map›Paper›PMID 37006762›Full record

ReviewJACS Au2023

Challenges and Perspectives of Single-Atom-Based Catalysts for Electrochemical Reactions.

Jiazhan Li, Chang Chen, Lekai Xu, Yu Zhang, Wei Wei, Erbo Zhao, Yue Wu, Chen Chen

Abstract readReview
In one paragraph

Review in JACS Au, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 24 papers.

0numbers the graph read from it
0cells of the map it votes in
24citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

24 citing papers in PubMed.

  1. Mixed-Valence Atomic-Layer Iridium Patches Enhance Alkaline Hydrogen Evolution.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026
    Article
  2. Article
  3. Bidirectional Soft Catalysts for Improved Power Performance of Li-S Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026
    Article
  4. Review
  5. Review
  6. Article
  7. Review
  8. Review
  9. Rigid Supramolecular Aramid Nanotubes as Catalyst Supports.Advanced materials (Deerfield Beach, Fla.) · 2026
    Article
  10. Article
  11. Review
  12. Review
  13. Review
  14. Article
  15. Article
  16. Unlocking COiScience · 2025
    Review
  17. Non-Aqueous Electrochemical COSmall (Weinheim an der Bergstrasse, Germany) · 2025
    Article
  18. MXene-Supported Single-Atom Electrocatalysts.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025
    Review
  19. Article
  20. Tunable NACS applied materials & interfaces · 2025
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Jiazhan LiEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Chang ChenEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Lekai XuEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.ORCID https://orcid.org/0000-0002-5792-9932
Yu ZhangEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Wei WeiEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Erbo ZhaoEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Yue WuEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.
Chen ChenEngineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P. R. China.ORCID https://orcid.org/0000-0001-5902-3037

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Single-atom catalysts (SACs) are emerging as the most promising catalysts for various electrochemical reactions. The isolated dispersion of metal atoms enables high density of active sites, and the simplified structure makes them ideal model systems to study the structure-performance relationships. However, the activity of SACs is still insufficient, and the stability of SACs is usually inferior but has received little attention, hindering their practical applications in real devices. Moreover, the catalytic mechanism on a single metal site is unclear, leading the development of SACs to rely on trial-and-error experiments. How can one break the current bottleneck of active sites density? How can one further increase the activity/stability of metal sites? In this Perspective, we discuss the underlying reasons for the current challenges and identify precisely controlled synthesis involving designed precursors and innovative heat-treatment techniques as the key for the development of high-performance SACs. In addition, advanced operando characterizations and theoretical simulations are essential for uncovering the true structure and electrocatalytic mechanism of an active site. Finally, future directions that may arise breakthroughs are discussed.

Identifiers

PMID37006762
PMCPMC10052268

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.