ArticleLangmuir : the ACS journal of surfaces and colloids2023
Surprising Use of the Business Innovation Bass Diffusion Model To Accurately Describe Adsorption Isotherm Types I, III, and V.
Article in Langmuir : the ACS journal of surfaces and colloids, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed.
- An adsorbate biased dynamic 3D porous framework for inverse COChemical science · 2024Article
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2 authors.
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Abstract
Using adsorption isotherm data to determine heats of adsorption or predict mixture adsorption using the ideal adsorbed solution theory (IAST) relies on accurate fits of the data with continuous, mathematical models. Here, we derive an empirical two-parameter model to fit isotherm data of IUPAC types I, III, and V in a descriptive way based on the Bass model for innovation diffusion. We report 31 isotherm fits to existing literature data covering all six types of isotherms, various adsorbents, such as carbons, zeolites, and metal-organic frameworks (MOFs), as well as different adsorbing gases (water, carbon dioxide, methane, and nitrogen). We find several cases, especially for flexible MOFs, where previously reported isotherm models reached their limits and either failed to fit the data or could not sufficiently be fitted due to stepped type V isotherms. Moreover, in two instances, models specifically developed for distinct systems are fitted with a higher
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