ArticleNature communications2023
The collective burst mechanism of angular jumps in liquid water.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Ferroelectricity in graphene nanoribbon devices enabled by collective water molecule dynamics.Nature communications · 2025Article
- Chain Formation and Addition Drive the Debye Relaxation of Methanol.The journal of physical chemistry. B · 2025Article
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- Spatiotemporal characterization of water diffusion anomalies in saline solutions using machine learning force field.Science advances · 2024Article
- Topological Frustration Triggers Ultrafast Dynamics of Monolayer Water Confined in Graphene Slit Pores.Nano letters · 2024Article
- Revisiting the Thickness of the Air-Water Interface from Two Extremes of Interface Hydrogen Bond Dynamics.Journal of chemical theory and computation · 2024Article
- Confinement Effects on Reorientation Dynamics of Water Confined within Graphite Nanoslits.The journal of physical chemistry. B · 2024Article
- How Thick is the Air-Water Interface?─A Direct Experimental Measurement of the Decay Length of the Interfacial Structural Anisotropy.Langmuir : the ACS journal of surfaces and colloids · 2024Article
- A new method to calculate broadband dielectric spectra of solvents from molecular dynamics simulations demonstrated with polarizable force fields.The Journal of chemical physics · 2024Article
- Evidence of ferroelectric features in low-density supercooled water from ab initio deep neural-network simulations.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Spontaneous Dipole Reorientation in Confined Water and Its Effect on Wetting/Dewetting of Hydrophobic Nanopores.ACS applied materials & interfaces · 2024Article
- Lessons Learned from Multiobjective Automatic Optimizations of Classical Three-Site Rigid Water Models Using Microscopic and Macroscopic Target Experimental Observables.Journal of chemical and engineering data · 2023Article
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Authors and funding
5 authors.
Funding
Abstract
Understanding the microscopic origins of collective reorientational motions in aqueous systems requires techniques that allow us to reach beyond our chemical imagination. Herein, we elucidate a mechanism using a protocol that automatically detects abrupt motions in reorientational dynamics, showing that large angular jumps in liquid water involve highly cooperative orchestrated motions. Our automatized detection of angular fluctuations, unravels a heterogeneity in the type of angular jumps occurring concertedly in the system. We show that large orientational motions require a highly collective dynamical process involving correlated motion of many water molecules in the hydrogen-bond network that form spatially connected clusters going beyond the local angular jump mechanism. This phenomenon is rooted in the collective fluctuations of the network topology which results in the creation of defects in waves on the THz timescale. The mechanism we propose involves a cascade of hydrogen-bond fluctuations underlying angular jumps and provides new insights into the current localized picture of angular jumps, and its wide use in the interpretations of numerous spectroscopies as well in reorientational dynamics of water near biological and inorganic systems. The role of finite size effects, as well as of the chosen water model, on the collective reorientation is also elucidated.
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