ArticleNature communications2023
Nanoarchitecture factors of solid electrolyte interphase formation via 3D nano-rheology microscopy and surface force-distance spectroscopy.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Article
- Atomic force nanorheology forFaraday discussions · 2026Article
- Unravelling friction anisotropy by atomic force microscopy.Journal of microscopy · 2026Review
- Modulated electrochemical force microscopy: Investigation of sodium-ion transport at hard carbon composite anodes.Journal of microscopy · 2026Article
- All-Atomic Computational Perspectives for Understanding Morphable Electric Double Layers: A Review.Small (Weinheim an der Bergstrasse, Germany) · 2025Review
- Atomic Force Microscopy for Cross-Disciplinary Materials Research.Small methods · 2025Review
- Advances in nanomechanical property mapping by atomic force microscopy.Nanoscale advances · 2025Review
- Resolving Nanoslip, Solvation Inertia, and Charge Dynamics at Vibrating Solid-Liquid Interface.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- In Situ Electrochemical Atomic Force Microscopy Study of Interfacial Reactions on a Graphite Negative Electrode for Magnesium-Ion Batteries.International journal of molecular sciences · 2025Article
- Nonlinear Harmonics: A Gateway to Enhanced Image Contrast and Material Discrimination.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Recent advances in characterization of rechargeable battery materialsJournal of materials chemistry. A · 2025Article
- Effect of the Formation Rate on the Stability of Anode-Free Lithium Metal Batteries.ACS energy letters · 2024Article
- Robust bilayer solid electrolyte interphase for Zn electrode with high utilization and efficiency.Nature communications · 2024Article
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Authors and funding
14 authors.
Funding
Abstract
The solid electrolyte interphase in rechargeable Li-ion batteries, its dynamics and, significantly, its nanoscale structure and composition, hold clues to high-performing and safe energy storage. Unfortunately, knowledge of solid electrolyte interphase formation is limited due to the lack of in situ nano-characterization tools for probing solid-liquid interfaces. Here, we link electrochemical atomic force microscopy, three-dimensional nano-rheology microscopy and surface force-distance spectroscopy, to study, in situ and operando, the dynamic formation of the solid electrolyte interphase starting from a few 0.1 nm thick electrical double layer to the full three-dimensional nanostructured solid electrolyte interphase on the typical graphite basal and edge planes in a Li-ion battery negative electrode. By probing the arrangement of solvent molecules and ions within the electric double layer and quantifying the three-dimensional mechanical property distribution of organic and inorganic components in the as-formed solid electrolyte interphase layer, we reveal the nanoarchitecture factors and atomistic picture of initial solid electrolyte interphase formation on graphite-based negative electrodes in strongly and weakly solvating electrolytes.
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