ReviewChemSusChem2023
Understanding and Engineering Interfacial Adhesion in Solid-State Batteries with Metallic Anodes.
Review in ChemSusChem, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
What it found
Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.
The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.
Who cites it
3 citing papers in PubMed, 30 citations in OpenAlex.
- Review
- Electro-chemo-mechanics of anode-free solid-state batteries.Nature materials · 2025Review
- Understanding and Engineering Interfacial Adhesion in Solid-State Batteries with Metallic Anodes.ChemSusChem · 2023Review
Corrections and comments
PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.
Authors and funding
5 authors at 2 institutions in 2 countries.
Funding
Abstract
High performance alkali metal anode solid-state batteries require solid/solid interfaces with fast ion transfer that are morphologically and chemically stable upon electrochemical cycling. Void formation at the alkali metal/solid-state electrolyte interface during alkali metal stripping is responsible for constriction resistances and hotspots that can facilitate dendrite propagation and failure. Both externally applied pressures (35-400 MPa) and temperatures above the melting point of the alkali metal have been shown to improve the interfacial contact with the solid electrolyte, preventing the formation of voids. However, the extreme pressure and temperature conditions required can be difficult to meet for commercial solid-state battery applications. In this review, we highlight the importance of interfacial adhesion or 'wetting' at alkali metal/solid electrolyte interfaces for achieving solid-state batteries that can withstand high current densities without cell failure. The intrinsically poor adhesion at metal/ceramic interfaces poses fundamental limitations on many inorganics solid-state electrolyte systems in the absence of applied pressure. Suppression of alkali metal voids can only be achieved for systems with high interfacial adhesion (i. e. 'perfect wetting') where the contact angle between the alkali metal and the solid-state electrolyte surface goes to θ=0°. We identify key strategies to improve interfacial adhesion and suppress void formation including the adoption of interlayers, alloy anodes and 3D scaffolds. Computational modeling techniques have been invaluable for understanding the structure, stability and adhesion of solid-state battery interfaces and we provide an overview of key techniques. Although focused on alkali metal solid-state batteries, the fundamental understanding of interfacial adhesion discussed in this review has broader applications across the field of chemistry and material science from corrosion to biomaterials development.
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What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.