ArticleNature communications2023
Entangled spin-polarized excitons from singlet fission in a rigid dimer.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 16 papers.
What it found
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The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
16 citing papers in PubMed, 45 citations in OpenAlex.
- Electron transfer from singlet fission dimers: possibilities and limitations.Chemical science · 2026Article
- An experimental perspective on symmetry breaking and the singlet fission mechanism in solid-state materials.Chemical science · 2026Review
- Single-Carbon Bridged Pentacene Dimers Enable Efficient Singlet Fission and Quintet State Stabilization.Journal of the American Chemical Society · 2026Article
- High-spin state dynamics and quintet-mediated emission in intramolecular singlet fission.Nature communications · 2026Article
- Enhancing the Optically Detected Magnetic Resonance Signal of Organic Molecular Qubits.ACS central science · 2025Article
- The Acetylene Bridge in Intramolecular Singlet Fission: A Boon or A Nuisance?Angewandte Chemie (International ed. in English) · 2024Article
- Theoretical Study on Singlet Fission Dynamics and Triplet Migration Process in Symmetric Heterotrimer Models.Molecules (Basel, Switzerland) · 2024Article
- Spin-bearing molecules as optically addressable platforms for quantum technologies.Nanophotonics (Berlin, Germany) · 2024Review
- The Interplay of Strongly and Weakly Exchange-Coupled Triplet Pairs in Intramolecular Singlet Fission.Journal of the American Chemical Society · 2024Article
- Tailoring Coherent Microwave Emission from a Solid-State Hybrid System for Room-Temperature Microwave Quantum Electronics.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Revealing the Singlet Fission Mechanism for a Silane-Bridged Thienotetracene Dimer.The journal of physical chemistry. A · 2024Article
- Enhancing NIR-to-visible upconversion in a rigidly coupled tetracene dimer: approaching statistical limits for triplet-triplet annihilation using intramolecular multiexciton states.Chemical science · 2024Article
- Room-temperature quantum coherence of entangled multiexcitons in a metal-organic framework.Science advances · 2024Article
- Molecular Control of Triplet-Pair Spin Polarization and Its Optoelectronic Magnetic Resonance Probes.Accounts of chemical research · 2024Article
- Multiexciton quintet state populations in a rigid pyrene-bridged parallel tetracene dimer.Chemical science · 2023Article
- Near-Infrared Absorption Features of Triplet-Pair States Assigned by Photoinduced-Absorption-Detected Magnetic Resonance.The journal of physical chemistry letters · 2023Article
Corrections and comments
PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.
Authors and funding
5 authors at 2 institutions in 1 country.
Funding
Abstract
Singlet fission, a process that splits a singlet exciton into a biexciton, has promise in quantum information. We report time-resolved electron paramagnetic resonance measurements on a conformationally well-defined acene dimer molecule, TIPS-BP1', designed to exhibit strongly state-selective relaxation to specific magnetic spin sublevels. The resulting optically pumped spin polarization is a nearly pure initial state from the ensemble. The long-lived spin coherences modulate the signal intrinsically, allowing a measurement scheme that substantially removes noise and uncertainty in the magnetic resonance spectra. A nonadiabatic transition theory with a minimal number of spectroscopic parameters allows the quantitative assignment and interpretation of the spectra. In this work, we show that the rigid dimer TIPS-BP1' supports persistent spin coherences at temperatures far higher than those used in conventional superconducting quantum hardware.
Identifiers
What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.