ArticleACS polymers Au2021
Terpyridine-Induced Folding of Anisotropic Polyphosphoester Platelets.
Article in ACS polymers Au, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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4 authors at 1 institution in 2 countries.
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Abstract
The folding of macromolecules is of great importance in nature. Also in synthetic polymer chemistry, single-chain nanoparticles, i.e. folding synthetic macromolecules, are a current research topic to mimic protein folding and to generate well-defined structures. Here, we present the "folding" of anisotropic polymer platelets to further mimic natural folding processes on the (sub)micrometer scale. We report on the synthesis of terpyridine-functionalized long-chain polyphosphoesters by acyclic diene metathesis polymerization that can crystallize in dilute solution into anisotropic polymer crystal platelets. As the terpyridine units are expelled to the platelet surface, terpyridine-metal interactions could be induced by adding nickel(II) bis(acetylacetonate) (Ni(acac)
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