ArticleInternational journal of molecular sciences2023
In-Situ Electrochemical Exfoliation and Methylation of Black Phosphorus into Functionalized Phosphorene Nanosheets.
Article in International journal of molecular sciences, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed, 22 citations in OpenAlex.
- Recent Advances and Critical Review on Two-Dimensional Black Phosphorus: Preparation and Optoelectronic Applications.Materials (Basel, Switzerland) · 2026Review
- Effect of covalent functionalisation with isocyanates on the electrochemical properties of exfoliated black phosphorus electrodes.Scientific reports · 2025Article
- Exploring the frontier: nonlinear optics in low dimensional materials.Nanophotonics (Berlin, Germany) · 2025Review
- Recent Advances in Novel Compositions for Electrochemical Applications.International journal of molecular sciences · 2023Article
- Covalent Functionalization of Black Phosphorus Nanosheets with Dichlorocarbenes for Enhanced Electrocatalytic Hydrogen Evolution Reaction.Nanomaterials (Basel, Switzerland) · 2023Article
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Authors and funding
12 authors at 4 institutions in 1 country.
Funding
Abstract
Two-dimensional black phosphorus (BP) has attracted great attention as a perspective material for various applications. The chemical functionalization of BP is an important pathway for the preparation of materials with improved stability and enhanced intrinsic electronic properties. Currently, most of the methods for BP functionalization with organic substrates require either the use of low-stable precursors of highly reactive intermediates or the use of difficult-to-manufacture and flammable BP intercalates. Herein we report a facile route for simultaneous electrochemical exfoliation and methylation of BP. Conducting the cathodic exfoliation of BP in the presence of iodomethane makes it possible to generate highly active methyl radicals, which readily react with the electrode's surface yielding the functionalized material. The covalent functionalization of BP nanosheets with the P-C bond formation has been proven by various microscopic and spectroscopic methods. The functionalization degree estimated by solid-state
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Registered trials
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