ArticleACS measurement science au2021
Accessing In Situ Photocorrosion under Realistic Light Conditions: Photoelectrochemical Scanning Flow Cell Coupled to Online ICP-MS.
Article in ACS measurement science au, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Chemistry of Materials Underpinning Photoelectrochemical Solar Fuel Production.Chemical reviews · 2025Review
- Key Aspects in Designing High-Throughput Workflows in Electrocatalysis Research: A Case Study on IrCo Mixed-Metal Oxides.ACS materials letters · 2024Article
- Scanning Gas Diffusion Electrode Setup for Real-Time Analysis of Catalyst Layers.ACS measurement science au · 2024Article
- Stability and degradation of (oxy)nitride photocatalysts for solar water splitting.RSC sustainability · 2024Review
- Interfacing High-Throughput Electrosynthesis and Mass Spectrometric Analysis of Azines.Analytical chemistry · 2024Article
- Article
- High-throughput exploration of activity and stability for identifying photoelectrochemical water splitting materials.Chemical science · 2022Article
Corrections and comments
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
High-impact photoelectrode materials for photoelectrochemical (PEC) water splitting are distinguished by synergistically attaining high photoactivity and stability at the same time. With numerous efforts toward optimizing the activity, the bigger challenge of tailoring the durability of photoelectrodes to meet industrially relevant levels remains. In situ photostability measurements hold great promise in understanding stability-related properties. Although different flow systems coupled to light-emitting diodes were introduced recently to measure time-resolved photocorrosion, none of the measurements were performed under realistic light conditions. In this paper, a photoelectrochemical scanning flow cell connected to an inductively coupled plasma mass spectrometer (PEC-ICP-MS) and equipped with a solar simulator, Air Mass 1.5 G filter, and monochromator was developed. The established system is capable of independently assessing basic PEC metrics, such as photopotential, photocurrent, incident photon to current efficiency (IPCE), and band gap in a high-throughput manner as well as the in situ photocorrosion behavior of photoelectrodes under standardized and realistic light conditions by coupling it to an ICP-MS. Polycrystalline platinum and tungsten trioxide (WO
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Registered trials
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