ArticleCommunications chemistry2020
Rapid access to discrete and monodisperse block co-oligomers from sugar and terpenoid toward ultrasmall periodic nanostructures.
Article in Communications chemistry, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Accessing Frank-Kasper Phases via Blending of Architecturally Distinct and Sustainable Sugar-Based Block Co-Oligomers.Macromolecules · 2025Article
- Targeting 2D Nanostructures in Phase-Separated Materials through Molecular Design.Macromolecules · 2025Article
- Crystal Lattice Analysis for 2D Nanomorphology Prediction of Phase-Separated Materials.Journal of the American Chemical Society · 2025Article
- Stereochemistry-dependent thermotropic liquid crystalline phases of monosaccharide-based amphiphiles.Soft matter · 2023Article
- Heating-Induced Switching to Hierarchical Liquid Crystallinity Combining Colloidal and Molecular Order in Zwitterionic Molecules.ACS omega · 2023Article
- Tunable Ordered Nanostructured Phases by Co-assembly of Amphiphilic Polyoxometalates and Pluronic Block Copolymers.Nano letters · 2023Article
- Fabrication of Ultrafine, Highly Ordered Nanostructures Using Carbohydrate-Inorganic Hybrid Block Copolymers.Nanomaterials (Basel, Switzerland) · 2022Article
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Authors and funding
12 authors.
Funding
Abstract
Discrete block co-oligomers (BCOs) are gaining considerable attention due to their potential to form highly ordered ultrasmall nanostructures suitable for lithographic templates. However, laborious synthetic routes present a major hurdle to the practical application. Herein, we report a readily available discrete BCO system that is capable of forming various self-assembled nanostructures with ultrasmall periodicity. Click coupling of propargyl-functionalized sugars (containing 1-7 glucose units) and azido-functionalized terpenoids (containing 3, 4, and 9 isoprene units) afforded the discrete and monodisperse BCOs with a desired total degree of polymerization and block ratio. These BCOs microphase separated into lamellar, gyroid, and cylindrical morphologies with the domain spacing (d) of 4.2-7.5 nm. Considering easy synthesis and rich phase behavior, presented BCO systems could be highly promising for application to diverse ~4-nm nanofabrications.
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