ArticleCommunications chemistry2022
A localized view on molecular dissociation via electron-ion partial covariance.
Article in Communications chemistry, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Photoinduced Enhancement of Chemical Shift Sensitivity to Local Vibrations.Journal of the American Chemical Society · 2026Article
- Wavelength-dependent photodissociation of iodomethylbutane.Scientific reports · 2025Article
- Conditional guided generative diffusion for particle accelerator beam diagnostics.Scientific reports · 2024Article
- The Role of Momentum Partitioning in Covariance Ion Imaging Analysis.The journal of physical chemistry. A · 2024Article
- Exploring the ultrafast and isomer-dependent photodissociation of iodothiophenesPhysical chemistry chemical physics : PCCP · 2024Article
- Theoretical study of time-resolved photoelectron circular dichroism in the photodissociation of a chiral molecule.Structural dynamics (Melville, N.Y.) · 2023Article
- Time-Resolved X-ray Photoelectron Spectroscopy: Ultrafast Dynamics in CSThe journal of physical chemistry letters · 2023Article
- Photoionization and Photofragmentation Dynamics of IThe journal of physical chemistry. A · 2022Article
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Authors and funding
40 authors.
Funding
Abstract
Inner-shell photoelectron spectroscopy provides an element-specific probe of molecular structure, as core-electron binding energies are sensitive to the chemical environment. Short-wavelength femtosecond light sources, such as Free-Electron Lasers (FELs), even enable time-resolved site-specific investigations of molecular photochemistry. Here, we study the ultraviolet photodissociation of the prototypical chiral molecule 1-iodo-2-methylbutane, probed by extreme-ultraviolet (XUV) pulses from the Free-electron LASer in Hamburg (FLASH) through the ultrafast evolution of the iodine 4d binding energy. Methodologically, we employ electron-ion partial covariance imaging as a technique to isolate otherwise elusive features in a two-dimensional photoelectron spectrum arising from different photofragmentation pathways. The experimental and theoretical results for the time-resolved electron spectra of the 4d
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