Evidence map›Paper›PMID 36658157›Full record

ArticleNature communications2023

Integrated interfacial design of covalent organic framework photocatalysts to promote hydrogen evolution from water.

Ting He, Wenlong Zhen, Yongzhi Chen, Yuanyuan Guo, Zhuoer Li, Ning Huang, Zhongping Li, Ruoyang Liu, Yuan Liu, Xu Lian and 4 more

Abstract read
In one paragraph

Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.

0numbers the graph read from it
0cells of the map it votes in
14citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

14 citing papers in PubMed.

  1. Article
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  5. Review
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  11. Article
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  13. Solar-Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024
    Review
  14. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

Ting HeDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Wenlong ZhenSchool of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore, 639798, Singapore.
Yongzhi ChenDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Yuanyuan GuoDivision of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore, 637371, Singapore.
Zhuoer LiDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Ning HuangMOE Key Laboratory of Macromolecular Synthesis and Functionalisation, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, 310027, China.ORCID http://orcid.org/0000-0002-7021-8705
Zhongping LiDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Ruoyang LiuDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Yuan LiuDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Xu LianDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Can XueSchool of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore, 639798, Singapore.
Tze Chien SumDivision of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore, 637371, Singapore.ORCID http://orcid.org/0000-0003-4049-2719
Wei ChenDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore.
Donglin JiangDepartment of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore, 117543, Singapore. chmjd@nus.edu.sg.ORCID http://orcid.org/0000-0002-3785-1330

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Attempts to develop photocatalysts for hydrogen production from water usually result in low efficiency. Here we report the finding of photocatalysts by integrated interfacial design of stable covalent organic frameworks. We predesigned and constructed different molecular interfaces by fabricating ordered or amorphous π skeletons, installing ligating or non-ligating walls and engineering hydrophobic or hydrophilic pores. This systematic interfacial control over electron transfer, active site immobilisation and water transport enables to identify their distinct roles in the photocatalytic process. The frameworks, combined ordered π skeletons, ligating walls and hydrophilic channels, work under 300-1000 nm with non-noble metal co-catalyst and achieve a hydrogen evolution rate over 11 mmol g

Identifiers

PMID36658157
PMCPMC9852592

What OpenQuestion holds

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LicenceCC BY
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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.