ArticleProceedings of the National Academy of Sciences of the United States of America2023
Mechanism for plasmon-generated solvated electrons.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed, 33 citations in OpenAlex.
- Quantum-Scale Friction at Solid-Liquid Interface: Simulation, Detection Techniques, Mechanisms, and Emerging Applications.Nano-micro letters · 2026Review
- Picosecond Stabilization of Transferred Charge Carriers at Plasmonic Metal-Molecule Interfaces.Angewandte Chemie (International ed. in English) · 2026Article
- Determination of the Generation Efficiency and Reductive Reactivity of the Upconverted Hot Electrons from Mn-Doped Quantum Dots under Weak Visible Light.Journal of the American Chemical Society · 2025Article
- Arrested Cooperative Electron Transfer by Stabilization of a Long-Lived Confined Unpaired Electron.JACS Au · 2025Article
- Alchemically-glazed plasmonic nanocavities using atomic layer metals: controllably synergizing catalysis and plasmonics.Nature communications · 2025Article
- Sustainable chemistry with plasmonic photocatalysts.Nanophotonics (Berlin, Germany) · 2023Review
Corrections and comments
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Authors and funding
16 authors at 1 institution in 1 country.
Funding
Abstract
Solvated electrons are powerful reducing agents capable of driving some of the most energetically expensive reduction reactions. Their generation under mild and sustainable conditions remains challenging though. Using near-ultraviolet irradiation under low-intensity one-photon conditions coupled with electrochemical and optical detection, we show that the yield of solvated electrons in water is increased more than 10 times for nanoparticle-decorated electrodes compared to smooth silver electrodes. Based on the simulations of electric fields and hot carrier distributions, we determine that hot electrons generated by plasmons are injected into water to form solvated electrons. Both yield enhancement and hot carrier production spectrally follow the plasmonic near-field. The ability to enhance solvated electron yields in a controlled manner by tailoring nanoparticle plasmons opens up a promising strategy for exploiting solvated electrons in chemical reactions.
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Registered trials
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