ArticleACS applied materials & interfaces2023
MOF-Polymer Mixed Matrix Membranes as Chemical Protective Layers for Solid-Phase Detoxification of Toxic Organophosphates.
Article in ACS applied materials & interfaces, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed, 44 citations in OpenAlex.
- Sodium alginate-based eco-friendly nanocomposites for textile wastewater management.RSC advances · 2026Review
- Bioengineered Ag/AgCl nanoparticles fromNanoscale advances · 2026Article
- MOF-decorated track-etched membranes for the U(VI) ions sorption removal.Scientific reports · 2025Article
- Synergistic Density Functional Theory and Molecular Dynamics Approach to Elucidate PNIPAM-Water Interaction Mechanisms.Materials (Basel, Switzerland) · 2025Article
- Modulated Optoelectronic Properties of MOF/CNF Bionanocomposite Films for Bacterial Growth Control under Visible Light.ACS applied materials & interfaces · 2025Article
- Proton Conduction in Zirconium-Based Metal-Organic Frameworks for Advanced Applications.ACS applied electronic materials · 2025Review
- Article
- Article
- Research Progress in the Degradation of Chemical Warfare Agent Simulants Using Metal-Organic Frameworks.Nanomaterials (Basel, Switzerland) · 2024Review
- MOFabric: an effective and wearable protective garment towards CWA detoxification.RSC advances · 2024Article
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Authors and funding
9 authors at 3 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Zirconium-based metal-organic frameworks (Zr-MOFs) have been demonstrated as potent catalysts for the hydrolytic detoxification of organophosphorus nerve agents and their simulants. However, the practical implementation of these Zr-MOFs is limited by the poor processability of their powdered form and the necessity of water media buffered by a volatile liquid base in the catalytic reaction. Herein, we demonstrate the efficient solid-state hydrolysis of a nerve agent simulant (dimethyl-4-nitrophenyl phosphate, DMNP) catalyzed by Zr-MOF-based mixed matrix membranes. The mixed matrix membranes were fabricated by incorporating MOF-808 into the blending matrix of poly(vinylidene fluoride) (PVDF), poly(vinylpyrrolidone) (PVP), and imidazole (Im), in which MOF-808 provides highly active catalytic sites, the hydrophilic PVP helps to retain water for promoting the hydrolytic reaction, and Im serves as a base for catalytic site regeneration. Impressively, the mixed matrix membranes displayed excellent catalytic performance for the solid-state hydrolysis of DMNP under high humidity, representing a significant step toward the practical application of Zr-MOFs in chemical protective layers against nerve agents.
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