ArticleAngewandte Chemie (International ed. in English)2023
Unimer Exchange Is not Necessary for Morphological Transitions in Polymerization-Induced Self-Assembly.
Article in Angewandte Chemie (International ed. in English), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Tuning the Length of Filomicelles Prepared Via Templated Polymerization-Induced Self-Assembly.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Leveraging Molecular Weight Dispersity for Scalable, Precise Synthesis of Nanocylinders Via Quasi-Polymerization-Induced Self-Assembly.Angewandte Chemie (International ed. in English) · 2026Article
- Kinetically Controlled and Nonequilibrium Assembly of Block Copolymers in Solution.Journal of the American Chemical Society · 2024Review
- Versatile morphology transition of nano-assemblies via ultrasonics/microwave assisted aqueous polymerization-induced self-assembly based on host-guest interaction.Ultrasonics sonochemistry · 2024Article
- Arginine-Functional Methacrylic Block Copolymer Nanoparticles: Synthesis, Characterization, and Adsorption onto a Model Planar Substrate.Biomacromolecules · 2024Article
- Preparation of diblock copolymer nano-assemblies by ultrasonics assisted ethanol-phase polymerization-induced self-assembly.Ultrasonics sonochemistry · 2024Article
- Unimer Exchange Is not Necessary for Morphological Transitions in Polymerization-Induced Self-Assembly.Angewandte Chemie (International ed. in English) · 2023Article
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7 authors.
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Abstract
Polymerization-induced self-assembly (PISA) has established itself as a powerful and straightforward method to produce polymeric nano-objects of various morphologies in (aqueous) solution. Generally, spheres are formed in the early stages of polymerization that may evolve to higher order morphologies (worms or vesicles), as the solvophobic block grows during polymerization. Hitherto, the mechanisms involved in these morphological transitions during PISA are still not well understood. Combining a systematic study of a representative PISA system with rheological measurements, we demonstrate that-unexpectedly-unimer exchange is not necessary to form higher order morphologies during radical RAFT-mediated PISA. Instead, in the investigated aqueous PISA, the monomer present in the polymerization medium is responsible for the morphological transitions, even though it slows down unimer exchange.
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