ArticleThe journal of physical chemistry. B2023
Correlated Fluctuations of Structural Indicators Close to the Liquid-Liquid Transition in Supercooled Water.
Article in The journal of physical chemistry. B, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed, 26 citations in OpenAlex.
- A local structural basis to distinguish amorphous ices.Nature communications · 2026Article
- Machine learning evaluation of structural descriptors for supercooled water.Communications chemistry · 2026Article
- Competing hydrogen-bond orders drive water's anomalous surface tension.Nature communications · 2026Article
- Direct observation of liquid-liquid phase coexistence in deeply supercooled water using an accurate polarizable multipole model.Proceedings of the National Academy of Sciences of the United States of America · 2026Article
- The interplay between liquid-liquid and ferroelectric phase transitions in supercooled water.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
Corrections and comments
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Authors and funding
2 authors at 2 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Multiple numerical studies have unambiguously shown the existence of a liquid-liquid critical point in supercooled states for different numerical models of water, and various structural indicators have been put forward to describe the transformation associated with this phase transition. Here we analyze numerical simulations of near-critical supercooled water to compare the behavior of several of such indicators with critical density fluctuations. We show that close to the critical point most indicators are strongly correlated to density, and some of them even display identical distributions of fluctuations. These indicators probe the exact same free energy landscape, therefore providing a thermodynamic description of critical supercooled water which is identical to that provided by the density order parameter. This implies that close to the critical point, there is a tight coupling between many, only apparently distinct, structural degrees of freedom.
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Registered trials
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