ArticleACS omega2022
Heat Generation and Degradation Mechanism of Lithium-Ion Batteries during High-Temperature Aging.
Article in ACS omega, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed, 96 citations in OpenAlex.
- Dual-Curved Cold-Plate Integration for Enhanced Liquid-Based Thermal Management of Cylindrical Li-Ion Batteries.ACS omega · 2026Article
- Faster and Durable: A Cell-to-System Validation of a Low-Degradation Fast-Charge Protocol for Li-Ion Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Low-Temperature Prediction in Commercial Lithium-Ion Batteries during Dynamic Usage via Enhanced Physics-Informed Neural Networks.ACS omega · 2026Article
- Thermal-electrical multiphysics modeling of ZnO/mesoporous carbon nanocomposite anodes for lithium-ion batteries.Scientific reports · 2026Article
- In Situ Liquid-Cell Transmission Electron Microscopy Insights Into Lithium-Ion Battery Materials Degradation: Challenges and Emerging Solutions.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- Thermal Modulation of Electrodeposition Stability in Sodium Metal Electrodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Structure-Tunable Fluorinated Polyester Electrolytes with Enhanced Interfacial Stability for Recyclable Solid-State Lithium Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- On-Site Portable Lithium Detection in Mining and Recycling Industries Based on a DNAzyme Fluorescent Sensor.Angewandte Chemie (International ed. in English) · 2025Article
- In Operando Optical Analysis of Electrolyte Colour Change and Its Correlation to Capacity Fade in Li-Ion Cells at Elevated Temperatures.Sensors (Basel, Switzerland) · 2024Article
- Glycerol Triacetate-Based Flame Retardant High-Temperature Electrolyte for the Lithium-Ion Battery.ACS applied materials & interfaces · 2024Article
Corrections and comments
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Authors and funding
5 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
High-temperature aging has a serious impact on the safety and performance of lithium-ion batteries. This work comprehensively investigates the evolution of heat generation characteristics upon discharging and electrochemical performance and the degradation mechanism during high-temperature aging. Post-mortem characterization analysis revealed that lithium plating is the main degradation mechanism. The occurrence of side reactions leads to cell capacity fading and electrochemical performance degradation. The DC resistance and AC impedance increase significantly, and the severe internal polarization makes the incremental capacity curve shift to lower voltage. In the early aging stage, the cell degrades slightly, and the temperature rise rate has not changed significantly upon discharging. The cell capacity plays a leading role, whose degradation makes the temperature rise decrease. With the aging deepening, the severe cell degradation makes the temperature rise rate increase significantly. Even if the capacity fading, the temperature rise still increases significantly compared to the fresh state. Furthermore, irreversible heat and reversible heat increase significantly with the aging deepening and current rate increasing.
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Registered trials
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