ArticleThe journal of physical chemistry letters2022
New Perspective on Electron Transfer through Molecules.
Article in The journal of physical chemistry letters, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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The trial behind it
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Who cites it
7 citing papers in PubMed.
- Engineering an Electrode-Electrolyte Interphase for Ultrastable Aqueous Aluminium-Air Battery.Angewandte Chemie (International ed. in English) · 2026Article
- An Orthogonal Electronic State View on Charge Delocalization and Transfer.The journal of physical chemistry. A · 2026Article
- A Nd@CNature · 2025Article
- What Can CISS Teach Us about Electron Transfer?The journal of physical chemistry letters · 2024Review
- Gradual Change between Coherent and Incoherent Tunneling Regimes Induced by Polarizable Halide Substituents in Molecular Tunnel Junctions.Journal of the American Chemical Society · 2024Article
- Current Induced Spin-Polarization in Chiral Molecules.The journal of physical chemistry letters · 2024Article
- Detection of a Chirality-Induced Spin Selective Quantum Capacitance in α-Helical Peptides.Nano letters · 2023Article
Corrections and comments
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Motivated by experiments which display unusual length and temperature effects for electron transfer in the nanometer length regime, we propose a new approach for describing long-range electron transfer (ET) processes through molecules. We posit that the electron reorganization in the molecules (e.g., the electronic polarization of a macromolecule or organic film by an applied electric potential, or the injected charge generating a dipole moment) should be included in the description. We numerically solve a one-dimensional model for the electron transport, which includes electron-electron interactions explicitly, and we show that it generates a power law distance dependence for electron transport similar to that observed in experiments. The model does not include vibrations explicitly and should be consistent with the weak temperature dependences observed experimentally. This approach emphasizes the need to treat the electronic changes in the molecule(s) more explicitly to understand the behavior.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.