ArticleScience advances2022
Eliminating interfacial O-involving degradation in Li-rich Mn-based cathodes for all-solid-state lithium batteries.
Article in Science advances, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 27 papers.
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Who cites it
27 citing papers in PubMed.
- Harnessing interfacial kosmotropic effect for reversible quasi-solid-state zinc-iodine batteries.Science advances · 2026Article
- Synthesis-Dependent Grain Boundary Density Governs Low-Temperature Lithium Diffusion in Single-Crystal NCM Cathodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Realizing long-cycling silicon-based all-solid-state batteries with near-zero-stress variation.Science advances · 2026Article
- Synergistic Regulation of Interfacial Potential and Anionic Covalency for High-Voltage Cobalt-Free All-Solid-State Batteries.Angewandte Chemie (International ed. in English) · 2026Article
- Thiourea-derived coating enabled lithium-rich manganese oxide positive electrode in solid-state batteries.Nature communications · 2026Article
- Synergistic interfacial-mechanical binder design for high-areal-capacity and long-lifespan Si-based negative electrodes in practical pouch cells.Nature communications · 2026Article
- Regulation Roles of p-Block Elements in Lithium Layered Oxide Cathodes: Recent Progress and Perspectives.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Interplay between oxygen redox and interfacial stability of Li-rich positive electrodes in sulfide-based all-solid-state batteries.Nature communications · 2026Article
- Anion-exchange fluorinated ion conductors for stable high-voltage lithium battery.Nature communications · 2026Article
- Modulating Lattice Oxygen and Transport Kinetics of Li-Rich Cathodes in All-Solid-State Batteries Through Multifunctional LiNano-micro letters · 2026Article
- Electrolyte-Induced Interfacial/Bulk Dual Regulation Enables Negligible Capacity Decay in Li-Rich Cathodes.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Optimizing Depth-of-Discharge in Li-Rich Halide All-Solid-State Batteries for Enhanced Capacity and Cycling Stability.Materials (Basel, Switzerland) · 2026Article
- Boosting LiNano-micro letters · 2026Review
- Space charge regulation for ultra-stable all-solid-state lithium batteries by engineering of argyrodite electrolyte.National science review · 2026Article
- Gradient-Modified Li-Rich Manganese-Based Oxides Cathodes with Breakthrough of Kinetic Limitation for High-Performance All-Solid-State Lithium Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Ligand-channel-induced ion liberation in crowded zwitterionic hydrogel electrolyte for efficient zinc metal batteries.Nature communications · 2025Article
- Enhancing the Cycling Stability of Amorphous-Based LiNiOACS nano · 2025Article
- Review on Cathode-Electrolyte Interphase for Stabilizing Interfaces in Solid-State Lithium Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Review
- Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries.Nature materials · 2025Article
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Authors and funding
12 authors.
Funding
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Abstract
In the pursuit of energy-dense all-solid-state lithium batteries (ASSBs), Li-rich Mn-based oxide (LRMO) cathodes provide an exciting path forward with unexpectedly high capacity, low cost, and excellent processibility. However, the cause for LRMO|solid electrolyte interfacial degradation remains a mystery, hindering the application of LRMO-based ASSBs. Here, we first reveal that the surface oxygen instability of LRMO is the driving force for interfacial degradation, which severely blocks the interfacial Li-ion transport and triggers fast battery failure. By replacing the charge compensation of surface oxygen with sulfite, the overoxidation and interfacial degradation can be effectively prevented, therefore achieving a high specific capacity (~248 mAh g
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Registered trials
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