Evidence map›Paper›PMID 36425339›Full record

ArticleACS earth & space chemistry2022

Effects of Atmospheric Aging Processes on Nascent Sea Spray Aerosol Physicochemical Properties.

Chathuri P Kaluarachchi, Victor W Or, Yiling Lan, Elias S Hasenecz, Deborah Kim, Chamika K Madawala, Glorianne P Dorcé, Kathryn J Mayer, Jonathan S Sauer, Christopher Lee and 6 more

Open access · hybridAbstract read
In one paragraph

Article in ACS earth & space chemistry, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.

0numbers the graph read from it
0cells of the map it votes in
8citing papers in PubMed
2.4field-weighted citation impact, top 11% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

8 citing papers in PubMed, 20 citations in OpenAlex.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

16 authors at 5 institutions in 1 country.

Chathuri P KaluarachchiDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.ORCID https://orcid.org/0000-0003-2538-3952
Victor W OrDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.
Yiling LanDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.
Elias S HaseneczDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.
Deborah KimDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.ORCID https://orcid.org/0000-0001-6717-8397
Chamika K MadawalaDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.
Glorianne P DorcéDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.
Kathryn J MayerDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.
Jonathan S SauerDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.
Christopher LeeScripps Institution of Oceanography, University of California, San Diego, La Jolla, California 92093, United States.
Christopher D CappaDepartment of Civil and Environmental Engineering, University of California, Davis, California 95616, United States.ORCID https://orcid.org/0000-0002-3528-3368
Timothy H BertramDepartment of Chemistry, University of Wisconsin-Madison, Madison, Wisconsin 53706, United States.
Elizabeth A StoneDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.ORCID https://orcid.org/0000-0003-0078-141X
Kimberly A PratherDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.
Vicki H GrassianDepartment of Chemistry and Biochemistry, University of California, San Diego, La Jolla, California 92093, United States.ORCID https://orcid.org/0000-0001-5052-0045
Alexei V TivanskiDepartment of Chemistry, University of Iowa, Iowa City, Iowa 52242, United States.ORCID https://orcid.org/0000-0002-1528-2421
University of Iowa · USUniversity of California San Diego · USScripps Institution of Oceanography · USUniversity of California, Davis · USUniversity of Wisconsin–Madison · US

Funding

Pulmonary Toxicology Facility CoreP30ES005605 · NIEHS · UNIVERSITY OF IOWA · PI Jong Sung Kim · 1990 to 2026
$40.5M
NIEHS NIH HHS P30 ES005605
6 · The paper itself

Abstract

The effects of atmospheric aging on single-particle nascent sea spray aerosol (nSSA) physicochemical properties, such as morphology, composition, phase state, and water uptake, are important to understanding their impacts on the Earth's climate. The present study investigates these properties by focusing on the aged SSA (size range of 0.1-0.6 μm) and comparing with a similar size range nSSA, both generated at a peak of a phytoplankton bloom during a mesocosm study. The aged SSAs were generated by exposing nSSA to OH radicals with exposures equivalent to 4-5 days of atmospheric aging. Complementary filter-based thermal optical analysis, atomic force microscopy (AFM), and AFM photothermal infrared spectroscopy were utilized. Both nSSA and aged SSA showed an increase in the organic mass fraction with decreasing particle sizes. In addition, aging results in a further increase of the organic mass fraction, which can be attributed to new particle formation and oxidation of volatile organic compounds followed by condensation on pre-existing particles. The results are consistent with single-particle measurements that showed a relative increase in the abundance of aged SSA core-shells with significantly higher organic coating thickness, relative to nSSA. Increased hygroscopicity was observed for aged SSA core-shells, which had more oxygenated organic species. Rounded nSSA and aged SSA had similar hygroscopicity and no apparent changes in the composition. The observed changes in aged SSA physicochemical properties showed a significant size-dependence and particle-to-particle variability. Overall, results showed that the atmospheric aging can significantly influence the nSSA physicochemical properties, thus altering the SSA effects on the climate.

Identifiers

PMID36425339
PMCPMC9677592
OpenAlexW4307391612

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.