Evidence map›Paper›PMID 36331392›Full record

ArticleNanoscale2022

Ionic dielectrics for fully printed carbon nanotube transistors: impact of composition and induced stresses.

Brittany N Smith, Hope Meikle, James L Doherty, Shiheng Lu, Gianna Tutoni, Matthew L Becker, Michael J Therien, Aaron D Franklin

Abstract read
In one paragraph

Article in Nanoscale, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Brittany N SmithDepartment of Electrical and Computer Engineering, Duke University, Durham, NC 27708, USA. aaron.franklin@duke.edu.ORCID http://orcid.org/0000-0003-2147-8735
Hope MeikleDepartment of Electrical and Computer Engineering, Duke University, Durham, NC 27708, USA. aaron.franklin@duke.edu.
James L DohertyDepartment of Electrical and Computer Engineering, Duke University, Durham, NC 27708, USA. aaron.franklin@duke.edu.ORCID http://orcid.org/0000-0003-1571-0622
Shiheng LuDepartment of Electrical and Computer Engineering, Duke University, Durham, NC 27708, USA. aaron.franklin@duke.edu.ORCID http://orcid.org/0000-0002-5323-7787
Gianna TutoniDepartment of Chemistry, Duke University, Durham, NC 27708, USA.
Matthew L BeckerDepartment of Chemistry, Duke University, Durham, NC 27708, USA.ORCID http://orcid.org/0000-0003-4089-6916
Michael J TherienDepartment of Chemistry, Duke University, Durham, NC 27708, USA.ORCID http://orcid.org/0000-0003-4876-0036
Aaron D FranklinDepartment of Electrical and Computer Engineering, Duke University, Durham, NC 27708, USA. aaron.franklin@duke.edu.ORCID http://orcid.org/0000-0002-1128-9327

Funding

Printed Electronic Biosensors for Point-of-Care Testing of Cardiovascular BiomarkersR01HL146849 · NHLBI · DUKE UNIVERSITY · PI FRANKLIN, AARON · 2019 to 2023
$2.6M
NHLBI NIH HHS R01 HL146849
6 · The paper itself

Abstract

Printed carbon nanotube thin-film transistors (CNT-TFTs) are candidates for flexible electronics with printability on a wide range of substrates. Among the layers comprising a CNT-TFT, the gate dielectric has proven most difficult to additively print owing to challenges in film uniformity, thickness, and post-processing requirements. Printed ionic dielectrics show promise for addressing these issues and yielding devices that operate at low voltages thanks to their high-capacitance electric double layers. However, the printing of ionic dielectrics in their various compositions is not well understood, nor is the impact of certain stresses on these materials. In this work, we studied three compositionally distinct ionic dielectrics in fully printed CNT-TFTs: the polar-fluorinated polymer elastomer PVDF-HFP; an ion gel consisting of triblock polymer PS-PMMA-PS and ionic liquid EMIM-TFSI; and crystalline nanocellulose (CNC) with a salt concentration of 0.05%. Although ion gel has been thoroughly studied, e-PVDF-HFP and CNC printing are relatively new and this study provides insights into their ink formulation, print processing, and performance as gate dielectrics. Using a consistent aerosol jet printing approach, each ionic dielectric was printed into similar CNT-TFTs, allowing for direct comparison through extensive characterization, including mechanical and electrical stress tests. The ionic dielectrics were found to have distinct operational dependencies based on their compositional and ionic attributes. Overall, the results reveal a number of trade-offs that must be managed when selecting a printable ionic dielectric, with CNC showing the strongest performance for low-voltage operation but the ion gel and elastomer exhibiting better stability under bias and mechanical stresses.

Identifiers

PMID36331392
PMCPMC9719746

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.