ReviewChemical communications (Cambridge, England)2022
Time-resolved X-ray and XUV based spectroscopic methods for nonadiabatic processes in photochemistry.
Review in Chemical communications (Cambridge, England), 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- A Theoretical Investigation of Nonadiabatic Dynamics and Time-Resolved NEXAFS Spectra of Uracil.ACS omega · 2026Article
- Simulation of time-resolved site-selective X-ray spectroscopy tracing nonadiabatic dynamics inPhysical chemistry chemical physics : PCCP · 2025Article
- Simulating nonadiabatic dynamics in benzophenone: Tracing internal conversion through photoelectron spectra.The Journal of chemical physics · 2025Article
- Raman Spectroscopy of Conical Intersections Using Entangled Photons.The journal of physical chemistry letters · 2024Article
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Authors and funding
4 authors.
Funding
Abstract
The photochemistry of numerous molecular systems is influenced by conical intersections (CIs). These omnipresent nonadiabatic phenomena provide ultra-fast radiationless relaxation channels by creating degeneracies between electronic states and decide over the final photoproducts. In their presence, the Born-Oppenheimer approximation breaks down, and the timescales of the electron and nuclear dynamics become comparable. Due to the ultra-fast dynamics and the complex interplay between nuclear and electronic degrees of freedom, the direct experimental observation of nonadiabatic processes close to CIs remains challenging. In this article, we give a theoretical perspective on novel spectroscopic techniques capable of observing clear signatures of CIs. We discuss methods that are based on ultra-short laser pulses in the extreme ultraviolet and X-ray regime, as their spectral and temporal resolution allow for resolving the ultra-fast dynamics near CIs.
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Registered trials
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