ArticleNature communications2022
Organic radicals stabilization above 300 °C in Eu-based coordination polymers for solar steam generation.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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Who cites it
7 citing papers in PubMed.
- Functional Metal Complexes for Solar-Light-Driven Energy Conversion.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Precise synthesis of π-conjugated [3]catenanes and Solomon link for photothermal responses via a dual-tuning strategy.Nature communications · 2026Article
- Systematic Tuning of the Electronic Effects in Covalent Organic Frameworks for Promoting Photocatalysis.ACS central science · 2025Article
- Deciphering a volcano-shaped relationship between radical stability and reticular electrochemiluminescence.Nature communications · 2025Article
- NIR-II photothermal conversion and imaging based on a cocrystal containing twisted components.Chemical science · 2024Article
- Stretchable photothermal membrane of NIR-II charge-transfer cocrystal for wearable solar thermoelectric power generation.Science advances · 2023Article
- Advancing Evidence-Based Data Interpretation in UV-Vis and Fluorescence Analysis for Nanomaterials: An Analytical Chemistry Perspective.Analytical chemistry · 2023Review
Corrections and comments
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Authors and funding
11 authors.
Funding
Abstract
Organic radicals feature unpaired electrons, and these compounds may have applications in biomedical technology and as materials for solar energy conversion. However, unpaired electrons tend to pair up (to form chemical bonds), making radicals unstable and hampering their applications. Here we report an organic radical system that is stable even at 350 °C, surpassing the upper temperature limit (200 °C) observed for other organic radicals. The system reported herein features a sulfur-rich organic linker that facilitates the formation of the radical centers; on the solid-state level, the molecules are crystallized with Eu(III) ions to form a 3D framework featuring stacks of linker molecules. The stacking is, however, somewhat loose and allows the molecules to wiggle and transform into sulfur-stabilized radicals at higher temperatures. In addition, the resulting solid framework remains crystalline, and it is stable to water and air. Moreover, it is black and features strong broad absorption in the visible and near IR region, thereby enhancing both photothermal conversion and solar-driven water evaporation.
Identifiers
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Registered trials
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