ArticleLangmuir : the ACS journal of surfaces and colloids2022
Liquid Heterostructures: Generation of Liquid-Liquid Interfaces in Free-Flowing Liquid Sheets.
Article in Langmuir : the ACS journal of surfaces and colloids, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed, 0 citations in OpenAlex.
- Surface structure of water from soft X-ray second harmonic generation.Nature communications · 2025Article
- A sub-100 nm thickness flat jet for extreme ultraviolet to soft X-ray absorption spectroscopy.Journal of synchrotron radiation · 2024Article
- 3D-printed sheet jet for stable megahertz liquid sample delivery at X-ray free-electron lasers.IUCrJ · 2023Article
- Thinner than a knife's edge: 3D-printed liquid sheet jet technology for solution phase XFEL experiments.IUCrJ · 2023Article
- Imaging temperature and thickness of thin planar liquid water jets in vacuum.Structural dynamics (Melville, N.Y.) · 2023Article
- Microfluidic liquid sheets as large-area targets for high repetition XFELs.Frontiers in molecular biosciences · 2022Article
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Authors and funding
6 authors at 3 institutions in 1 country.
Funding
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Abstract
Chemical reactions and biological processes are frequently governed by the structure and dynamics of the interface between two liquid phases, but these interfaces are often difficult to study due to the relative abundance of the bulk liquids. Here, we demonstrate a method for generating multilayer thin film stacks of liquids, which we call liquid heterostructures. These free-flowing layered liquid sheets are produced with a microfluidic nozzle that impinges two converging jets of one liquid onto opposite sides of a third jet of another liquid. The resulting sheet consists of two layers of the first liquid enveloping an inner layer of the second liquid. Infrared microscopy, white light reflectivity, and imaging ellipsometry measurements demonstrate that the buried liquid layer has a tunable thickness and displays well-defined liquid-liquid interfaces and that this inner layer can be only tens of nanometers thick. The demonstrated multilayer liquid sheets minimize the amount of bulk liquid relative to their buried interfaces, which makes them ideal targets for spectroscopy and scattering experiments.
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Registered trials
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