ArticleNature communications2022
Sub-optical-cycle light-matter energy transfer in molecular vibrational spectroscopy.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
What it found
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Who cites it
4 citing papers in PubMed.
- Tunable Plasmon-Enhanced Wide-Angle Terahertz Perfect Absorption via Lorentz Media.Nanophotonics (Berlin, Germany) · 2026Article
- Electric-Field Molecular Fingerprinting to Probe Cancer.ACS central science · 2025Article
- Standardized Electric-Field-Resolved Molecular Fingerprinting.Analytical chemistry · 2024Article
- Optical Force of Bessel Pincer Light-Sheets Beam on a Dielectric Sphere of Arbitrary Size.Nanomaterials (Basel, Switzerland) · 2022Article
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Authors and funding
6 authors.
Funding
Abstract
The evolution of ultrafast-laser technology has steadily advanced the level of detail in studies of light-matter interactions. Here, we employ electric-field-resolved spectroscopy and quantum-chemical modelling to precisely measure and describe the complete coherent energy transfer between octave-spanning mid-infrared waveforms and vibrating molecules in aqueous solution. The sub-optical-cycle temporal resolution of our technique reveals alternating absorption and (stimulated) emission on a few-femtosecond time scale. This behaviour can only be captured when effects beyond the rotating wave approximation are considered. At a femtosecond-to-picosecond timescale, optical-phase-dependent coherent transients and the dephasing of the vibrations of resonantly excited methylsulfonylmethane (DMSO
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Registered trials
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