ArticlePolymer chemistry2022
Influence of the molecular weight and size distribution of PSS on mixed ionic-electronic transport in PEDOT:PSS.
Article in Polymer chemistry, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed, 52 citations in OpenAlex.
- Transient Charging of Mixed Ionic-Electronic Conductors by Anomalous Diffusion.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- PEDOT: PSS for Implantable and Wearable Bioelectronics: From Material Engineering and Energy Storage to Clinical Translation.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Electrothermally Regenerable PEDOT:PSS/PVA Composite Films for Solid-State Dehumidification Applications.ACS omega · 2026Article
- Revealing the Full Potential of Glycolated Mixed Ionic-Electronic Semiconductors - Symmetric Monomer Polymerization to Boost Electrochemical Transistor Performance.Journal of the American Chemical Society · 2026Article
- Dose-Dependent, Biomechanical Recovery of Permeability Ex Vivo in GAG-Depleted Cartilage With a Synthetic Polyelectrolyte, Polystyrene Sulfonate.Journal of orthopaedic research : official publication of the Orthopaedic Research Society · 2026Article
- Enhanced Diffusion and Retention of Proteoglycan Replacements in Cartilage through Thermoresponsive Polyelectrolytes.Macromolecules · 2025Article
- Biomolecule Functionalization of Poly(3,4-ethylenedioxythiophene) Surfaces via Thiol-Maleimide Click-Chemistry.Chemistry of materials : a publication of the American Chemical Society · 2025Article
- Contorted acene ribbons for stable and ultrasensitive neural probes.Science advances · 2025Article
- Recent Advances in the Tunable Optoelectromagnetic Properties of PEDOTs.Molecules (Basel, Switzerland) · 2025Review
- Kinetics and Retention of Polystyrenesulfonate for Proteoglycan Replacement in Cartilage.Biomacromolecules · 2024Article
- Article
- Organic Electrochemical Transistors for Biomarker Detections.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Review
- 3D Printing Highly Efficient Ion-Exchange Materials via a Polyelectrolyte Microphase Separation Strategy.Small science · 2024Article
- One Pot Photomediated Formation of Electrically Conductive Hydrogels.ACS polymers Au · 2024Article
- Influence of protonic acid on the structure and properties of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) in oxidation polymerization.RSC advances · 2024Article
- Surface Functionalization with (3-Glycidyloxypropyl)trimethoxysilane (GOPS) as an Alternative to Blending for Enhancing the Aqueous Stability and Electronic Performance of PEDOT:PSS Thin Films.ACS applied materials & interfaces · 2023Article
- Design of Microstructure-Engineered Polymers for Energy and Environmental Conservation.JACS Au · 2023Review
- On the fundamentals of organic mixed ionic/electronic conductors.Journal of materials chemistry. C · 2023Article
Corrections and comments
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Authors and funding
11 authors at 3 institutions in 1 country.
Funding
Abstract
The commercially available polyelectrolyte complex poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) is ubiquitous in organic and hybrid electronics. As such, it has often been used as a benchmark material for fundamental studies and the development of new electronic devices. Yet, most studies on PEDOT:PSS have focused on its electronic conductivity in dry environments, with less consideration given to its ion transport, coupled ionic-electronic transport, and charge storage properties in aqueous environments. These properties are essential for applications in bioelectronics (sensors, actuators), charge storage devices, and electrochromic displays. Importantly, past studies on mixed ionic-electronic transport in PEDOT:PSS neglected to consider how the molecular structure of PSS affects mixed ionic-electronic transport. Herein, we therefore investigated the effect of the molecular weight and size distribution of PSS on the electronic properties and morphology of PEDOT:PSS both in dry and aqueous environments, and overall performance in organic electrochemical transistors (OECTs). Using reversible addition-fragmentation chain transfer (RAFT) polymerization with two different chain transfer agents, six PSS samples with monomodal, narrow (
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.