ArticleChemical science2022
Surface coverage control for dramatic enhancement of thermal CO oxidation by precise potential tuning of metal supported catalysts.
Article in Chemical science, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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3 citing papers in PubMed.
- Positive Electrochemical Potentials Induce Enhanced Chemoselectivity and Activity in the Thermocatalytic Hydrogenation of 3-Nitrostyrene.Angewandte Chemie (International ed. in English) · 2026Article
- Bridging mixed potential theory and electrochemical promotion of thermal catalysis during hydroquinone-benzoquinone redox reactions.Nature communications · 2025Article
- Potential-Rate Correlations of Supported Palladium-Based Catalysts for Aqueous Formic Acid Dehydrogenation.Journal of the American Chemical Society · 2024Article
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Authors and funding
6 authors.
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Abstract
Chemical heterogeneous catalysis maximizes performance by controlling the interactions between the catalyst and the substrates. Steady-state catalytic rates depend on the heat of adsorption and the resultant coverage of adsorbates, which in turn reflects the electronic structure of the heterogeneous catalyst surfaces. This study aims to free the surface from high coverage of a kind of substance by externally controlling the electrochemical potential of the catalysts for improved thermal-catalytic rates. We employed aqueous CO oxidation at 295 K as a model reaction, where strong binding of chemisorbed CO (CO*) to the metal surfaces and its high coverage led to inhibition of O
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