Evidence map›Paper›PMID 36065004›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2022

Charge-Compensated N-Doped π-Conjugated Polymers: Toward both Thermodynamic Stability of N-Doped States in Water and High Electron Conductivity.

Fabian Borrmann, Takuya Tsuda, Olga Guskova, Nataliya Kiriy, Cedric Hoffmann, David Neusser, Sabine Ludwigs, Uwe Lappan, Frank Simon, Martin Geisler and 4 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

Fabian BorrmannLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.
Takuya TsudaLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.
Olga GuskovaLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0001-5925-6586
Nataliya KiriyLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.
Cedric HoffmannLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.
David NeusserIPOC-Functional Polymers, Institute of Polymer Chemistry & Center for Integrated Quantum Science and Technology (IQST), University of Stuttgart, Pfaffenwaldring 55, 70569, Stuttgart, Germany.
Sabine LudwigsIPOC-Functional Polymers, Institute of Polymer Chemistry & Center for Integrated Quantum Science and Technology (IQST), University of Stuttgart, Pfaffenwaldring 55, 70569, Stuttgart, Germany.
Uwe LappanLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0002-7464-9449
Frank SimonLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0002-4063-1742
Martin GeislerLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0002-9414-0914
Bipasha DebnathLeibniz-Institut für Festkörper- und Werkstoffforschung Dresden, Helmholtzstraße 20, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0002-8562-1994
Yulia KrupskayaLeibniz-Institut für Festkörper- und Werkstoffforschung Dresden, Helmholtzstraße 20, 01069, Dresden, Germany.
Mahmoud Al-HusseinPhysics Department and Hamdi Mango Center for Scientific Research, The University of Jordan, Amman, 11942, Jordan.ORCID https://orcid.org/0000-0002-4395-6833
Anton KiriyLeibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069, Dresden, Germany.ORCID https://orcid.org/0000-0002-4263-9377

Funding

Carl Zeiss Foundation IQSTDFG GU1510/5-1DFG KR4364/4European Social Fund 100235479
6 · The paper itself

Abstract

The understanding and applications of electron-conducting π-conjugated polymers with naphtalene diimide (NDI) blocks show remarkable progress in recent years. Such polymers demonstrate a facilitated n-doping due to the strong electron deficiency of the main polymer chain and the presence of the positively charged side groups stabilizing a negative charge of the n-doped backbone. Here, the n-type conducting NDI polymer with enhanced stability of its n-doped states for prospective "in-water" applications is developed. A combined experimental-theoretical approach is used to identify critical features and parameters that control the doping and electron transport process. The facilitated polymer reduction ability and the thermodynamic stability in water are confirmed by electrochemical measurements and doping studies. This material also demonstrates a high conductivity of 10

Indexed as

density functional theory calculationselectron conductivityn-doped statesthermodynamic stabilityπ-conjugated polymers

Identifiers

PMID36065004
PMCPMC9631074

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.