ArticleChemistry of materials : a publication of the American Chemical Society2022
Nucleation of Porous Crystals from Ion-Paired Prenucleation Clusters.
Article in Chemistry of materials : a publication of the American Chemical Society, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Electro-assisted control over zeolite crystallization and modification: theory, configuration, and applications.Journal of materials chemistry. A · 2026Review
- Ion exchange selectivity governs phase selection in zeolite synthesis.Materials horizons · 2025Article
- Design Principles Of Inorganic-Protein Hybrid Materials for Biomedicine.Exploration (Beijing, China) · 2025Review
- Illuminating the Black Box: A Perspective on Zeolite Crystallization in Inorganic Media.Accounts of chemical research · 2023Article
- Does Water Enable Porosity in Aluminosilicate Zeolites? Porous Frameworks versus Dense Minerals.Crystal growth & design · 2023Article
- Structural Aspects Affecting Phase Selection in Inorganic Zeolite Synthesis.Chemistry of materials : a publication of the American Chemical Society · 2022Article
- HSIL-Based Synthesis of Ultracrystalline K,Na-JBW, a Zeolite Exhibiting Exceptional Framework Ordering and Flexibility.Chemistry of materials : a publication of the American Chemical Society · 2022Article
- Ion-Pairs in Aluminosilicate-Alkali Synthesis Liquids Determine the Aluminum Content and Topology of Crystallizing Zeolites.Chemistry of materials : a publication of the American Chemical Society · 2022Article
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Authors and funding
12 authors.
Funding
Abstract
Current nucleation models propose manifold options for the formation of crystalline materials. Exploring and distinguishing between different crystallization pathways on the molecular level however remain a challenge, especially for complex porous materials. These usually consist of large unit cells with an ordered framework and pore components and often nucleate in complex, multiphasic synthesis media, restricting in-depth characterization. This work shows how aluminosilicate speciation during crystallization can be documented in detail in monophasic hydrated silicate ionic liquids (HSILs). The observations reveal that zeolites can form via supramolecular organization of ion-paired prenucleation clusters, consisting of aluminosilicate anions, ion-paired to alkali cations, and imply that zeolite crystallization from HSILs can be described within the spectrum of modern nucleation theory.
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