ArticleChemical science2022
Ni single atoms on carbon nitride for visible-light-promoted full heterogeneous dual catalysis.
Article in Chemical science, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Single-Atom Site Photocatalysts Boosting Organic Synthesis: The Integration of a Metal Active Site and Photosensitive Unit.Nanomaterials (Basel, Switzerland) · 2026Review
- Selective Semi-Hydrogenation of Acetylene using a Single-Atom Cobalt on Carbon Nitride Photocatalyst with Water as a Proton Source.Small methods · 2026Article
- General method for carbon-heteroatom cross-coupling reactions via semiheterogeneous red-light metallaphotocatalysis.Nature communications · 2025Article
- An Adaptive Palladium Single-Atom Catalyst Enabling Reactivity Switching between Borylation and C-C Coupling.Journal of the American Chemical Society · 2025Article
- Resolving the Nanostructure of Carbon Nitride-Supported Single-Atom Catalysts.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Structure-activity relationships in the development of single atom catalysts for sustainable organic transformations.Nanoscale advances · 2025Review
- Cu Anchored Carbon Nitride (Cu/CN) Catalyzes Selective Oxidation of Thiol by Controlling Reactive Oxygen Species Generation.ACS nano · 2024Article
- Nickel atom-clusters nanozyme for boosting ferroptosis tumor therapy.Materials today. Bio · 2024Article
- Electrostatic [FeFe]-hydrogenase-carbon nitride assemblies for efficient solar hydrogen production.Chemical science · 2024Article
- Programmable Photocatalytic Activity of Multicomponent Covalent Organic Frameworks Used as Metallaphotocatalysts.Chemistry (Weinheim an der Bergstrasse, Germany) · 2023Article
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Authors and funding
17 authors.
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Abstract
Visible-light-driven organic transformations are of great interest in synthesizing valuable fine chemicals under mild conditions. The merger of heterogeneous photocatalysts and transition metal catalysts has recently drawn much attention due to its versatility for organic transformations. However, these semi-heterogenous systems suffered several drawbacks, such as transition metal agglomeration on the heterogeneous surface, hindering further applications. Here, we introduce heterogeneous single Ni atoms supported on carbon nitride (NiSAC/CN) for visible-light-driven C-N functionalization with a broad substrate scope. Compared to a semi-heterogeneous system, high activity and stability were observed due to metal-support interactions. Furthermore, through systematic experimental mechanistic studies, we demonstrate that the stabilized single Ni atoms on CN effectively change their redox states, leading to a complete photoredox cycle for C-N coupling.
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