Evidence map›Paper›PMID 35941110›Full record

ArticleNature communications2022

Development of high-energy non-aqueous lithium-sulfur batteries via redox-active interlayer strategy.

Byong-June Lee, Chen Zhao, Jeong-Hoon Yu, Tong-Hyun Kang, Hyean-Yeol Park, Joonhee Kang, Yongju Jung, Xiang Liu, Tianyi Li, Wenqian Xu and 4 more

Open access · goldAbstract read
In one paragraph

Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.

0numbers the graph read from it
0cells of the map it votes in
8citing papers in PubMed
8.9field-weighted citation impact, top 1% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

8 citing papers in PubMed, 101 citations in OpenAlex.

  1. Review
  2. Article
  3. Recent Advances on Transition Metal Sulfides for Key Components of Lithium-Sulfur Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025
    Review
  4. Article
  5. Review
  6. Article
  7. Article
  8. Li-S Chemistry of Manganese Phosphides Nanoparticles With Optimized Phase.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors at 4 institutions in 3 countries.

Byong-June Lee *Department of Energy Science and Engineering, Daegu Gyeongbuk Institute of Science & Technology (DGIST), Daegu, 42988, Republic of Korea.
Chen Zhao *Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US.
Jeong-Hoon YuDepartment of Energy Science and Engineering, Daegu Gyeongbuk Institute of Science & Technology (DGIST), Daegu, 42988, Republic of Korea.
Tong-Hyun KangDepartment of Energy Science and Engineering, Daegu Gyeongbuk Institute of Science & Technology (DGIST), Daegu, 42988, Republic of Korea.ORCID http://orcid.org/0000-0003-4292-2110
Hyean-Yeol ParkDepartment of Energy Science and Engineering, Daegu Gyeongbuk Institute of Science & Technology (DGIST), Daegu, 42988, Republic of Korea.
Joonhee KangDepartment of Nanoenergy Engineering, Pusan National University, Busan, 46241, Republic of Korea.
Yongju JungDepartment of Chemical Engineering, Korea University of Technology and Education (KOREATECH), Cheonan, 330-708, Republic of Korea.
Xiang LiuChemical Sciences and Engineering Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US.ORCID http://orcid.org/0000-0003-3293-9373
Tianyi LiX-ray Science Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US.ORCID http://orcid.org/0000-0002-6234-6096
Wenqian XuX-ray Science Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US.
Xiao-Bing ZuoX-ray Science Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US.ORCID http://orcid.org/0000-0002-0134-4804
Gui-Liang XuChemical Sciences and Engineering Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US. xug@anl.gov.ORCID http://orcid.org/0000-0001-9969-883X
Khalil AmineChemical Sciences and Engineering Division, Argonne National Laboratory, 9700S Cass Ave, Lemont, IL, 60439, US. amine@anl.gov.ORCID http://orcid.org/0000-0001-9206-3719
Jong-Sung YuDepartment of Energy Science and Engineering, Daegu Gyeongbuk Institute of Science & Technology (DGIST), Daegu, 42988, Republic of Korea. jsyu@dgist.ac.kr.ORCID http://orcid.org/0000-0002-8805-012X
Argonne National Laboratory · USDaegu Gyeongbuk Institute of Science and Technology · KRKorea University of Technology and Education · KRPusan National University · KR

Funding

National Research Foundation of Korea (NRF) 2016M1A2A2937137National Research Foundation of Korea (NRF) 2019R1A2C2086770U.S. Department of Energy (DOE) DE-AC02-06CH11357
6 · The paper itself

Abstract

Lithium-sulfur batteries have theoretical specific energy higher than state-of-the-art lithium-ion batteries. However, from a practical perspective, these batteries exhibit poor cycle life and low energy content owing to the polysulfides shuttling during cycling. To tackle these issues, researchers proposed the use of redox-inactive protective layers between the sulfur-containing cathode and lithium metal anode. However, these interlayers provide additional weight to the cell, thus, decreasing the practical specific energy. Here, we report the development and testing of redox-active interlayers consisting of sulfur-impregnated polar ordered mesoporous silica. Differently from redox-inactive interlayers, these redox-active interlayers enable the electrochemical reactivation of the soluble polysulfides, protect the lithium metal electrode from detrimental reactions via silica-polysulfide polar-polar interactions and increase the cell capacity. Indeed, when tested in a non-aqueous Li-S coin cell configuration, the use of the interlayer enables an initial discharge capacity of about 8.5 mAh cm

Identifiers

PMID35941110
PMCPMC9360432
OpenAlexW4291021285

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.