ReviewEnergy & fuels : an American Chemical Society journal2021
Recent Advances and Perspectives in Photodriven Charge Accumulation in Molecular Compounds: A Mini Review.
Review in Energy & fuels : an American Chemical Society journal, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
What it found
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Who cites it
12 citing papers in PubMed.
- Light-Driven Proton-Coupled Two-Electron Ligand Reduction Causes the Rearrangement of the Coordination Sphere in Cu(I) 4Journal of the American Chemical Society · 2026Article
- Unveiling the Light Induced Energy Transfer Events in Water Soluble Benzothiazole Appended Borondipyrromethene: Synthesis, Photophysical Study, and Applications to Amyloid Binding.Chemistry, an Asian journal · 2026Article
- Photoinduced double charge accumulation in a molecular compound.Nature chemistry · 2025Article
- Unveiling photoinduced electron transfers in photosensitized polyoxometalates for solar energy conversion.Chemical science · 2025Review
- Molecular Design Principles for Achieving High-Efficiency Light-Induced Charge Separation at the Nanometer Scale.JACS Au · 2025Article
- Arrested Cooperative Electron Transfer by Stabilization of a Long-Lived Confined Unpaired Electron.JACS Au · 2025Article
- Photoinduced ultrafast multielectron transfer and long-lived charge-accumulated state in a fullerene-indacenodithiophene dumbbell triad.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- From Molecular to Polymeric Donors: Prolonged Charge Separation in Modular Photoredox-Active Ru(II) Polypyridyl-Type Triads.Inorganic chemistry · 2024Article
- Photochemical charge accumulation in a heteroleptic copper(i)-anthraquinone molecular dyadChemical science · 2023Article
- Better Covalent Connection in a Molecular Triad Enables More Efficient Photochemical Energy Storage.Inorganic chemistry · 2023Article
- Accumulation of Four Electrons on a Terphenyl (Bis)disulfide.Chemistry (Weinheim an der Bergstrasse, Germany) · 2022Article
- Photophysics of Perylene Diimide Dianions and Their Application in Photoredox Catalysis.Angewandte Chemie (International ed. in English) · 2022Article
Corrections and comments
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Authors and funding
2 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The formation of so-called solar fuels from abundant low-energetic compounds, such as carbon dioxide or water, relies on the chemical elementary steps of photoinduced electron transfer and accumulation of multiple redox equivalents. The majority of molecular systems explored to date require sacrificial electron donors to accumulate multiple electrons on a single acceptor unit, but the use of high-energetic sacrificial redox reagents is unsustainable. In recent years, an increasing number of molecular compounds for reversible light-driven accumulation of redox equivalents that do not need sacrificial electron donors has been reported. Those compounds are the focus of this mini review. Different concepts, such as redox potential compression (achieved by proton-coupled electron transfer, Lewis acid-base interactions, or structural rearrangements), hybrids with inorganic nanoparticles, and diffusion-controlled multi-component systems, will be discussed. Newly developed strategies to outcompete unproductive reaction pathways in favor of desired photoproduct formation will be compared, and the importance of identifying reaction intermediates in the course of multiphotonic excitation by different time-resolved spectroscopic techniques will be discussed. The mechanistic insights gained from molecular donor-photosensitizer-acceptor compounds inform the design of next-generation charge accumulation systems for solar energy conversion.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.