ArticleScience advances2022
Designing broadband pulsed dynamic nuclear polarization sequences in static solids.
Article in Science advances, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Symmetry-based pulsed DNP and EPR sequences.Science advances · 2026Article
- In situ learning-based spin engineering of pulsed dynamic nuclear polarization.Science advances · 2026Article
- High-frequency dynamic nuclear polarization in rotating solids.Science advances · 2026Review
- Characterization of strongly hyperfine-split protons by DNP.Physical chemistry chemical physics : PCCP · 2026Article
- Effective Hamiltonian-Based DNP Sequence Optimization.The journal of physical chemistry letters · 2026Article
- Dynamic Nuclear Polarization with P1 Centers in Diamond.The journal of physical chemistry letters · 2024Article
- Observation of dynamic nuclear polarization echoes.Science advances · 2024Article
- Pulsed dynamic nuclear polarization: a comprehensive Floquet description.Physical chemistry chemical physics : PCCP · 2024Article
- Frequency-swept dynamic nuclear polarization.Journal of magnetic resonance (San Diego, Calif. : 1997) · 2023Article
- Coherent Dynamic Nuclear Polarization using Chirped Pulses.The journal of physical chemistry letters · 2023Article
- Reverse dynamic nuclear polarisation for indirect detection of nuclear spins close to unpaired electrons.Magnetic resonance (Gottingen, Germany) · 2022Article
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Dynamic nuclear polarization (DNP) is a nuclear magnetic resonance (NMR) hyperpolarization technique that mediates polarization transfer from unpaired electrons with large thermal polarization to NMR-active nuclei via microwave (mw) irradiation. The ability to generate arbitrarily shaped mw pulses using arbitrary waveform generators allows for remarkable improvement of the robustness and versatility of DNP. We present here novel design principles based on single-spin vector effective Hamiltonian theory to develop new broadband DNP pulse sequences, namely, an adiabatic version of XiX (X-inverse X)-DNP and a broadband excitation by amplitude modulation (BEAM)-DNP experiment. We demonstrate that the adiabatic BEAM-DNP pulse sequence may achieve a
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.