ArticleNature communications2022
Decoupled temperature and pressure hydrothermal synthesis of carbon sub-micron spheres from cellulose.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed, 182 citations in OpenAlex.
- Small Sample Machine Learning for Predicting Composition Changes in Chemically Pretreated Kapok Fiber.ACS omega · 2026Article
- Ion Compensation-Assisted Photolithography Enables High-Resolution Electrolytes for Neuromorphic Transistors.Nano-micro letters · 2026Article
- Hydrothermal Humification of Biomass for Circular Carbon Management in Sustainable Agro-Ecosystems.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- Biomass-Derived Carbon Quantum Dots via Semi-Hydrothermal Processing: Linking Surface Chemistry, Colloidal Stability, and Photocatalytic Mineralization Performance.Nanomaterials (Basel, Switzerland) · 2026Article
- Integrated hydrochar-bacteria strategy for heavy metal removal.Frontiers in microbiology · 2026Review
- Enhancing carbon-negative emission technologies through biomass integration.Innovation (Cambridge (Mass.)) · 2025Review
- Elastic Deformation of Cellulose/Lignin-Based Anode for Rejuvenating Aged Mix-Cultured Electroactive Biofilms.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Magnetic-Field-Induced Spin Transition in Single-Atom Catalysts for Nitrate Electrolysis to Ammonia.Nano letters · 2025Article
- Co-hydrothermal carbonization of pretreated sludge and polyethylene terephthalate for the preparation of low-nitrogen clean solid fuels.RSC advances · 2024Article
- Characterization of sago tree parts from Sentani, Papua, Indonesia for biomass energy utilization.Heliyon · 2024Article
- Van Krevelen diagrams based on machine learning visualize feedstock-product relationships in thermal conversion processes.Communications chemistry · 2023Article
- Article
- The Application of Biochar for COIndustrial & engineering chemistry research · 2023Article
- Review
- Cellulose Nanocrystal Embedded Composite Foam and Its Carbonization for Energy Application.Polymers · 2023Article
- Reduction of Hexavalent Chromium from Soil of the Relocated Factory Area with Rice Straw Hydrothermal Carbon Modified by Nano Zero-Valent Iron (nZVI).International journal of environmental research and public health · 2023Article
- Biomass-Based Hydrothermal Carbons for the Contaminants Removal of Wastewater: A Mini-Review.International journal of molecular sciences · 2023Review
- Preparation of tobacco pyrolysis liquids in subcritical/supercritical ethanol and their application in the aroma enhancement of heated cigarettes.Frontiers in chemistry · 2023Article
Corrections and comments
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Authors and funding
10 authors at 4 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The temperature and pressure of the hydrothermal process occurring in a batch reactor are typically coupled. Herein, we develop a decoupled temperature and pressure hydrothermal system that can heat the cellulose at a constant pressure, thus lowering the degradation temperature of cellulose significantly and enabling the fast production of carbon sub-micron spheres. Carbon sub-micron spheres can be produced without any isothermal time, much faster compared to the conventional hydrothermal process. High-pressure water can help to cleave the hydrogen bonds in cellulose and facilitate dehydration reactions, thus promoting cellulose carbonization at low temperatures. A life cycle assessment based on a conceptual biorefinery design reveals that this technology leads to a substantial reduction in carbon emissions when hydrochar replacing fuel or used for soil amendment. Overall, the decoupled temperature and pressure hydrothermal treatment in this study provides a promising method to produce sustainable carbon materials from cellulose with a carbon-negative effect.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.