ArticleNature communications2022
Effect of the grain arrangements on the thermal stability of polycrystalline nickel-rich lithium-based battery cathodes.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
6 citing papers in PubMed.
- Elemental Tuning of NMC Cathode Materials: Atomic Structural Variations Drive Performance Improvements.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Demonstrating Faster Multi-Label Grey-Level Analysis for Crack Detection in Ex Situ and Operando Micro-CT Images of NMC Electrode.Small methods · 2025Article
- Revealing the Chemical and Structural Complexity of Electrochemical Ion Exchange in Layered Oxide Materials.Journal of the American Chemical Society · 2024Article
- Direct Regeneration of Spent Lithium-Ion Battery Cathodes: From Theoretical Study to Production Practice.Nano-micro letters · 2024Review
- Enabling Electrochemical-Mechanical Robustness of Ultra-High Ni Cathode via Self-Supported Primary-Grain-Alignment Strategy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Surface coating by mechanofusion modulates bulk charging pathways and battery performance of Ni-rich layered cathodes.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
Corrections and comments
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Authors and funding
10 authors.
Funding
Abstract
One of the most challenging aspects of developing high-energy lithium-based batteries is the structural and (electro)chemical stability of Ni-rich active cathode materials at thermally-abused and prolonged cell cycling conditions. Here, we report in situ physicochemical characterizations to improve the fundamental understanding of the degradation mechanism of charged polycrystalline Ni-rich cathodes at elevated temperatures (e.g., ≥ 40 °C). Using multiple microscopy, scattering, thermal, and electrochemical probes, we decouple the major contributors for the thermal instability from intertwined factors. Our research work demonstrates that the grain microstructures play an essential role in the thermal stability of polycrystalline lithium-based positive battery electrodes. We also show that the oxygen release, a crucial process during battery thermal runaway, can be regulated by engineering grain arrangements. Furthermore, the grain arrangements can also modulate the macroscopic crystallographic transformation pattern and oxygen diffusion length in layered oxide cathode materials.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.