Evidence map›Paper›PMID 35694333›Full record

ArticleChemical science2022

Probing emission of a DNA-stabilized silver nanocluster from the sub-nanosecond to millisecond timescale in a single measurement.

Mikkel Baldtzer Liisberg, Stefan Krause, Cecilia Cerretani, Tom Vosch

Abstract read
In one paragraph

Article in Chemical science, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.

0numbers the graph read from it
0cells of the map it votes in
12citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

12 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Review
  5. Article
  6. Article
  7. Article
  8. Interrupted DNA and Slow Silver Cluster Luminescence.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023
    Article
  9. Chloride Ligands on DNA-Stabilized Silver Nanoclusters.Journal of the American Chemical Society · 2023
    Article
  10. Excited-State Dynamics in a DNA-Stabilized AgThe journal of physical chemistry letters · 2023
    Article
  11. Article
  12. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

4 authors.

Mikkel Baldtzer LiisbergNanoscience Center, Department of Chemistry, University of Copenhagen Universitetsparken 5 2100 Copenhagen Denmark tom@chem.ku.dk.ORCID https://orcid.org/0000-0001-7623-5453
Stefan KrauseNanoscience Center, Department of Chemistry, University of Copenhagen Universitetsparken 5 2100 Copenhagen Denmark tom@chem.ku.dk.ORCID https://orcid.org/0000-0002-7062-8472
Cecilia CerretaniNanoscience Center, Department of Chemistry, University of Copenhagen Universitetsparken 5 2100 Copenhagen Denmark tom@chem.ku.dk.ORCID https://orcid.org/0000-0002-3048-5438
Tom VoschNanoscience Center, Department of Chemistry, University of Copenhagen Universitetsparken 5 2100 Copenhagen Denmark tom@chem.ku.dk.ORCID https://orcid.org/0000-0001-5435-2181

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

A method for measuring emission over a range of sub-nanosecond to millisecond timescales is presented and demonstrated for a DNA-stabilized silver nanocluster (DNA-AgNC) displaying dual emission. This approach allows one to disentangle the temporal evolution of the two spectrally overlapping signals and to determine both the nano- and microsecond decay times of the two emission components, together with the time they take to reach the steady-state equilibrium. Addition of a second near-infrared laser, synchronized with a fixed delay, enables simultaneous characterization of optically activated delayed fluorescence (OADF). For this particular DNA-AgNC, we demonstrate that the microsecond decay times of the luminescent state and the OADF-responsible state are similar, indicating that the OADF process starts from the luminescent state.

Identifiers

PMID35694333
PMCPMC9116328

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.