ArticleNature communications2022
High-resolution two-dimensional electronic spectroscopy reveals the homogeneous line profile of chromophores solvated in nanoclusters.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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4 citing papers in PubMed.
- Selective Q‑Band Excitation Modulates Exciton-Exciton Annihilation in Tetra(ACS physical chemistry Au · 2026Article
- Gas-Phase Electronic Structure of Phthalocyanine Ions: A Study of Symmetry and Solvation Effects.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Unifying Nonlinear Response and Incoherent Mixing in Action-2D Electronic Spectroscopy.The journal of physical chemistry letters · 2023Article
- Dimer photofragmentation and cation ejection dynamics in helium nanodroplets.Physical chemistry chemical physics : PCCP · 2022Article
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3 authors.
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Abstract
Doped clusters in the gas phase provide nanoconfined model systems for the study of system-bath interactions. To gain insight into interaction mechanisms between chromophores and their environment, the ensemble inhomogeneity has to be lifted and the homogeneous line profile must be accessed. However, such measurements are very challenging at the low particle densities and low signal levels in cluster beam experiments. Here, we dope cryogenic rare-gas clusters with phthalocyanine molecules and apply action-detected two-dimensional electronic spectroscopy to gain insight into the local molecule-cluster environment for solid and superfluid cluster species. The high-resolution homogeneous linewidth analysis provides a benchmark for the theoretical modelling of binding configurations and shows a promising route for high-resolution molecular two-dimensional spectroscopy.
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