ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2022
Tuning 4f-Center Electron Structure by Schottky Defects for Catalyzing Li Diffusion to Achieve Long-Term Dendrite-Free Lithium Metal Battery.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Lanthanide Orbital Modulation Coupled With Entropy Increase Effect for Synergistically Enhanced Interfacial Stability and Ion Transport Kinetics in Halide Electrolytes.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Revitalizing dendritic lithium with atomic modulator-decorated suspension electrolyte for durable lithium metal batteries.Science advances · 2026Article
- Taming Interfacial Ion-Dipole Interactions With d-Orbital Delocalized Electron Catalysis Expediates Low-Temperature Li Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Suspension Electrolytes with Catalytically Self-Expediating Desolvation Kinetics for Low-Temperature Zinc Metal Batteries.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Low-Temperature Lithium Metal Batteries Achieved by Synergistically Enhanced Screening LiAdvanced materials (Deerfield Beach, Fla.) · 2025Article
- Tuning 4f-Center Electron Structure by Schottky Defects for Catalyzing Li Diffusion to Achieve Long-Term Dendrite-Free Lithium Metal Battery.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2022Article
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Authors and funding
13 authors.
Funding
Abstract
Lithium metal is considered as the most prospective electrode for next-generation energy storage systems due to high capacity and the lowest potential. However, uncontrollable spatial growth of lithium dendrites and the crack of solid electrolyte interphase still hinder its application. Herein, Schottky defects are motivated to tune the 4f-center electronic structures of catalysts to provide active sites to accelerate Li transport kinetics. As experimentally and theoretically confirmed, the electronic density is redistributed and affected by the Schottky defects, offering numerous active catalytic centers with stronger ion diffusion capability to guide the horizontal lithium deposition against dendrite growth. Consequently, the Li electrode with artificial electronic-modulation layer remarkably decreases the barriers of desolvation, nucleation, and diffusion, extends the dendrite-free plating lifespan up to 1200 h, and improves reversible Coulombic efficiency. With a simultaneous catalytic effect on the conversions of sulfur species at the cathodic side, the integrated Li-S full battery exhibits superior rate performance of 653 mA h g
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