ArticleNature communications2022
Unraveling the mechanism for paired electrocatalysis of organics with water as a feedstock.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
What it found
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Who cites it
18 citing papers in PubMed.
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- Photoelectrochemical valorisation of organic waste for the cogeneration of solar fuels and value-added chemicals.Chemical science · 2025Review
- Strong dipole-promoted N-O bond hydrogenolysis enables ampere-level electrosynthesis of methylamine.Nature chemistry · 2025Article
- MXene-Assisted NiFe sulfides for high-performance anion exchange membrane seawater electrolysis.Nature communications · 2025Article
- Porous N-Doped Carbon-encapsulated Iron as Novel Catalyst Architecture for the Electrocatalytic Hydrogenation of Benzaldehyde.ChemSusChem · 2025Article
- Synergistic enhancement of electrochemical alcohol oxidation by combining NiV-layered double hydroxide with an aminoxyl radical.Nature communications · 2025Article
- Parameterization and quantification of two key operando physio-chemical descriptors for water-assisted electro-catalytic organic oxidation.Nature communications · 2024Article
- A self-reactivated PdCu catalyst for aldehyde electro-oxidation with anodic hydrogen production.Nature communications · 2024Article
- Integrated electrochemical and chemical system for ampere-level production of terephthalic acid alternatives and hydrogen.Nature communications · 2024Article
- Enhanced electrocatalytic biomass oxidation at low voltage by NiNature communications · 2024Article
- Combining anodic alcohol oxidative coupling for C-C bond formation with cathodic ammonia production.National science review · 2024Article
- Paired electrocatalysis unlocks cross-dehydrogenative coupling of C(spNature communications · 2024Article
- Electrochemical hydrogenation and oxidation of organic species involving water.Nature reviews. Chemistry · 2024Review
- Electrocatalytic conversion of biomass-derived furan compounds: mechanisms, catalysts and perspectives.Chemical science · 2024Review
- Atomically dispersed Cu coordinated Rh metallene arrays for simultaneously electrochemical aniline synthesis and biomass upgrading.Nature communications · 2023Article
- Advances in Selective Electrochemical Oxidation of 5-Hydroxymethylfurfural to Produce High-Value Chemicals.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Review
- Recent Progress in Electrochemical Upgrading of Bio-Oil Model Compounds and Bio-Oils to Renewable Fuels and Platform Chemicals.Materials (Basel, Switzerland) · 2023Review
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Paired electroreduction and electrooxidation of organics with water as a feedstock to produce value-added chemicals is meaningful. A comprehensive understanding of reaction mechanism is critical for the catalyst design and relative area development. Here, we have systematically studied the mechanism of the paired electroreduction and electrooxidation of organics on Fe-Mo-based phosphide heterojunctions. It is shown that active H* species for organic electroreduction originate from water. As for organic electrooxidation, among various oxygen species (OH*, OOH*, and O*), OH* free radicals derived from the first step of water dissociation are identified as active species. Furthermore, explicit reaction pathways and their paired advantages are proposed based on theoretical calculations. The paired electrolyzer powered by a solar cell shows a low voltage of 1.594 V at 100 mA cm
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.