ArticleNature communications2022
Solution-processable microporous polymer platform for heterogenization of diverse photoredox catalysts.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Tailoring polymers of intrinsic microporosity as photoredox catalysts for continuous-flow reaction-separation processes.Nature communications · 2026Article
- Amination-degradation of super engineering plastics for the construction of surface emissive resin materials.Communications chemistry · 2026Article
- Combining Breath Figures with Mussel-Inspired Chemistry: An Easy Route to Finely Tunable Microporous Functional Surfaces.ACS materials Au · 2026Article
- Photoactive PFA Coating through Fluorophilic Interactions for Continuous Flow Photochemistry.JACS Au · 2025Article
- Heterogeneous organophotocatalytic HBr oxidation coupled with oxygen reduction for boosting bromination of arenes.Nature communications · 2024Article
- Recyclable and Stable Porphyrin-Based Self-Assemblies by Electrostatic Force for Efficient Photocatalytic Organic Transformation.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Heterogeneous Organocatalysts for Light-Driven Reactions in Continuous Flow.Molecules (Basel, Switzerland) · 2024Review
- Quantifying Förster Resonance Energy Transfer from Single Perovskite Quantum Dots to Organic Dyes.ACS nano · 2024Article
- Solution-processable polymers of intrinsic microporosity for gas-phase carbon dioxide photoreduction.Nature communications · 2023Article
- Porous Polymers Containing Metallocalix[4]arene for the Extraction of Tobacco-Specific Nitrosamines.Chemistry of materials : a publication of the American Chemical Society · 2022Article
- Hairy Conjugated Microporous Polymer Nanoparticles Facilitate Heterogeneous Photoredox Catalysis with Solvent-Specific Dispersibility.ACS nano · 2022Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
In contemporary organic synthesis, substances that access strongly oxidizing and/or reducing states upon irradiation have been exploited to facilitate powerful and unprecedented transformations. However, the implementation of light-driven reactions in large-scale processes remains uncommon, limited by the lack of general technologies for the immobilization, separation, and reuse of these diverse catalysts. Here, we report a new class of photoactive organic polymers that combine the flexibility of small-molecule dyes with the operational advantages and recyclability of solid-phase catalysts. The solubility of these polymers in select non-polar organic solvents supports their facile processing into a wide range of heterogeneous modalities. The active sites, embedded within porous microstructures, display elevated reactivity, further enhanced by the mobility of excited states and charged species within the polymers. The independent tunability of the physical and photochemical properties of these materials affords a convenient, generalizable platform for the metamorphosis of modern photoredox catalysts into active heterogeneous equivalents.
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