ArticleNature communications2022
Shape and structural relaxation of colloidal tactoids.
Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Remodeling and self-healing of individual amyloid tactoids via multiphoton absorption.Nature communications · 2025Article
- Confinement-driven structural transitions in a dusty plasma crystal.Scientific reports · 2025Article
- Functional Biomaterials Derived from Protein Liquid-Liquid Phase Separation and Liquid-to-Solid Transition.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Solvent-Dependent Dynamics of Cellulose Nanocrystals in Process-Relevant Flow Fields.Langmuir : the ACS journal of surfaces and colloids · 2024Article
- Structural Color from Cellulose Nanocrystals or Chitin Nanocrystals: Self-Assembly, Optics, and Applications.Chemical reviews · 2023Review
- Thermodynamically controlled multiphase separation of heterogeneous liquid crystal colloids.Nature communications · 2023Article
- Disentangling kinetics from thermodynamics in heterogeneous colloidal systems.Nature communications · 2023Article
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Authors and funding
5 authors.
Funding
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Abstract
Facile geometric-structural response of liquid crystalline colloids to external fields enables many technological advances. However, the relaxation mechanisms for liquid crystalline colloids under mobile boundaries remain still unexplored. Here, by combining experiments, numerical simulations and theory, we describe the shape and structural relaxation of colloidal liquid crystalline micro-droplets, called tactoids, where amyloid fibrils and cellulose nanocrystals are used as model systems. We show that tactoids shape relaxation bears a universal single exponential decay signature and derive an analytic expression to predict this out of equilibrium process, which is governed by liquid crystalline anisotropic and isotropic contributions. The tactoids structural relaxation shows fundamentally different paths, with first- and second-order exponential decays, depending on the existence of splay/bend/twist orientation structures in the ground state. Our findings offer a comprehensive understanding on dynamic confinement effects in liquid crystalline colloidal systems and may set unexplored directions in the development of novel responsive materials.
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