Evidence map›Paper›PMID 35545620›Full record

ArticleNature communications2022

Asymmetric electron acceptor enables highly luminescent organic solar cells with certified efficiency over 18.

Chengliang He, Zeng Chen, Tonghui Wang, Ziqiu Shen, Yaokai Li, Jiadong Zhou, Jianwei Yu, Huiyu Fang, Yuhao Li, Shuixing Li and 9 more

Abstract read
In one paragraph

Article in Nature communications, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 27 papers.

0numbers the graph read from it
0cells of the map it votes in
27citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

27 citing papers in PubMed.

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  16. Tackling Energy Loss in Organic Solar Cells via Volatile Solid Additive Strategy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

19 authors.

Chengliang He *State Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China.
Zeng Chen *Department of Chemistry, Zhejiang University, 310027, Hangzhou, P.R. China.
Tonghui Wang *Department of Chemistry and Biochemistry, The University of Arizona, Tucson, AR, 85721-0088, USA.
Ziqiu ShenState Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China.
Yaokai LiState Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China.
Jiadong ZhouInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, 510640, Guangzhou, P.R. China.
Jianwei YuDepartment of Physics, Chemistry, and Biology, Linköping University, Linköping, SE-58183, Sweden.
Huiyu FangState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, 710049, Xi'an, P.R. China.
Yuhao LiDepartment of Physics, Chinese University of Hong Kong, New Territories, 999077, Hong Kong, P. R. China.
Shuixing LiState Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China.
Xinhui LuDepartment of Physics, Chinese University of Hong Kong, New Territories, 999077, Hong Kong, P. R. China.ORCID http://orcid.org/0000-0002-1908-3294
Wei MaState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, 710049, Xi'an, P.R. China.
Feng GaoDepartment of Physics, Chemistry, and Biology, Linköping University, Linköping, SE-58183, Sweden.
Zengqi XieInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, 510640, Guangzhou, P.R. China.
Veaceslav CoropceanuDepartment of Chemistry and Biochemistry, The University of Arizona, Tucson, AR, 85721-0088, USA. coropceanu@arizona.edu.ORCID http://orcid.org/0000-0003-1693-2315
Haiming ZhuDepartment of Chemistry, Zhejiang University, 310027, Hangzhou, P.R. China. hmzhu@zju.edu.cn.ORCID http://orcid.org/0000-0001-7747-9054
Jean-Luc BredasDepartment of Chemistry and Biochemistry, The University of Arizona, Tucson, AR, 85721-0088, USA.ORCID http://orcid.org/0000-0001-7278-4471
Lijian ZuoState Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China. zjuzlj@zju.edu.cn.ORCID http://orcid.org/0000-0003-0338-1198
Hongzheng ChenState Key Laboratory of Silicon Materials, MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, 310027, Hangzhou, P.R. China. hzchen@zju.edu.cn.ORCID http://orcid.org/0000-0002-5922-9550

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Enhancing the luminescence property without sacrificing the charge collection is one key to high-performance organic solar cells (OSCs), while limited by the severe non-radiative charge recombination. Here, we demonstrate efficient OSCs with high luminescence via the design and synthesis of an asymmetric non-fullerene acceptor, BO-5Cl. Blending BO-5Cl with the PM6 donor leads to a record-high electroluminescence external quantum efficiency of 0.1%, which results in a low non-radiative voltage loss of 0.178 eV and a power conversion efficiency (PCE) over 15%. Importantly, incorporating BO-5Cl as the third component into a widely-studied donor:acceptor (D:A) blend, PM6:BO-4Cl, allows device displaying a high certified PCE of 18.2%. Our joint experimental and theoretical studies unveil that more diverse D:A interfacial conformations formed by asymmetric acceptor induce optimized blend interfacial energetics, which contributes to the improved device performance via balancing charge generation and recombination.

Identifiers

PMID35545620
PMCPMC9095617

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.